Thermoelastic equation of state of boron suboxide B6O up to 6 GPa and 2700 K: Simplified Anderson-Grüneisen model and thermodynamic ... View Full Text


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Article Info

DATE

2014-07

AUTHORS

O. O. Kurakevych, V. L. Solozhenko

ABSTRACT

The p-V-T equation of state of superhard boron suboxide B6O has been measured up to 6 GPa and 2700 K using multianvil technique and synchrotron X-ray diffraction. To fit the experimental data, the theoretical p-V-T equation of state has been derived in approximation of the constant value of the Anderson-Grüneisen parameter δT. Bulk modulus B0 =181 GPa and its first pressure derivative B0′ = 6 at 300 K; two parameters describing thermal expansion at 0.1 MPa, i.e., a = 1.4 × 10−5 K−1 and b = 5 × 10−9 K−2 as well as δT = 6 have been included in the model. The good agreement between fitted and experimental isobars has been achieved to the absolute volume changes up to 5% as compared to the volume at standard conditions, V0. The fitted thermal expansion at 0.1 MPa well consistent with the experimental data as well as with ambient-pressure heat capacity cp, bulk modulus B0 and δT describing its evolution with volume and temperature have been discussed. The fitted value of Grüneisen parameter γ = 0.85 in agreement with previous empiric estimations for B6O and experimental values for other boron-rich solids has been reported. More... »

PAGES

270-278

References to SciGraph publications

  • 2008-02. On the hardness of boron (III) oxide in JOURNAL OF SUPERHARD MATERIALS
  • 1993-01. A thermodynamic theory of the Grüneisen ratio at extreme conditions: MgO as an example in PHYSICS AND CHEMISTRY OF MINERALS
  • 2002-09-02. New materials from high-pressure experiments in NATURE MATERIALS
  • 2013-08-05. Equilibrium p-T Phase Diagram of Boron: Experimental Study and Thermodynamic Analysis in SCIENTIFIC REPORTS
  • 1987-06. High-pressure synthesis of B2O with diamond-like structure in JOURNAL OF MATERIALS SCIENCE LETTERS
  • 2010-06. Thermodynamic model of hardness: Particular case of boron-rich solids in JOURNAL OF SUPERHARD MATERIALS
  • 1998-01. Icosahedral packing of B12 icosahedra in boron suboxide (B6O) in NATURE
  • 2011-12-28. Mechanical properties and hardness of boron and boron-rich solids in JOURNAL OF SUPERHARD MATERIALS
  • 2003-09. Structural transformations in liquid, crystalline, and glassy B2O3 under high pressure in JETP LETTERS
  • 1987. Icosahedral Boron-Rich Solids as Refractory Semiconductors in MRS ADVANCES
  • 1993-01-01. Structure of B6O boron-suboxide by Rietveld refinement in JOURNAL OF MATERIALS SCIENCE
  • 2009-05-10. Investigation of polyamorphism in compressed B2O3 glass by the direct measurement of the density in JETP LETTERS
  • 2011-12-28. Experimental study and critical review of structural, thermodynamic and mechanical properties of superhard refractory boron suboxide B6O in JOURNAL OF SUPERHARD MATERIALS
  • 2009-06-28. Superhard phases of simple substances and binary compounds of the B-C-N-O system: from diamond to the latest results (a Review) in JOURNAL OF SUPERHARD MATERIALS
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    http://scigraph.springernature.com/pub.10.3103/s1063457614040054

    DOI

    http://dx.doi.org/10.3103/s1063457614040054

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    173 rdf:type schema:Organization
     




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