Plasmonic nanocavity enhanced luminescence for in-plane and out-of-plane excitons in BA2PbI4 Ruddlesden Popper perovskite thin film View Full Text


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Article Info

DATE

2022-04-06

AUTHORS

Yashika Gupta, Anuj K. Singh, Abhay Anand V. S., Anshuman Kumar

ABSTRACT

In this work, we propose an easy-to-fabricate plasmonic cavity design to enhance luminescence from BA2PbI4\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${\text{BA}}_{2} {\text{PbI}}_{4}$$\end{document} Ruddlesden Popper thin films, which otherwise suffer from a very low quantum yield due to strong exciton-phonon interactions in the lattice. We designed a nanoparticle on mirror plasmonic cavity using 3D-finite-difference time-domain simulations, with perovskite film sandwiched between the two metallic structures yielding a 7-fold local enhancement in photoluminescence for intralayer excitons emitting at 520 nm. The designed cavity also aids the detection of interlayer excitons at 540 nm, for which a huge PL enhancement of more than 1500 times is easily obtained.Graphical abstract More... »

PAGES

1-7

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URI

http://scigraph.springernature.com/pub.10.1557/s43580-022-00272-9

DOI

http://dx.doi.org/10.1557/s43580-022-00272-9

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https://app.dimensions.ai/details/publication/pub.1146923437


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