C60 and U ion irradiation of Gd2TixZr2−xO7 pyrochlore View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2015-08-28

AUTHORS

Jiaming Zhang, Marcel Toulemonde, Maik Lang, Jean Marc Costantini, Serge Della-Negra, Rodney C. Ewing

ABSTRACT

Gd 2 Ti x Zr 2− x O 7 ( x = 0 to 2) pyrochlore was irradiated by 30 MeV C 60 clusters, which provide an extremely high ionizing energy density. High-resolution transmission electron microscopy revealed a complex ion-track structure in Gd 2 Ti 2 O 7 and Gd 2 TiZrO 7 , consisting of an amorphous core and a shell of a disordered, defect-fluorite structure. As compared with the irradiation by 1.5 GeV U ions with the highest energy loss, the track structure is consistent with tracks created by monoatomic swift heavy ions, but the diameters (with the entire diameter of 17 nm for Gd 2 Ti 2 O 7 and 15 nm for Gd 2 TiZrO 7 ) are significantly larger due to the much smaller velocity and higher energy density of the C 60 ions. Ion tracks created by monoatomic ions are challenging to describe by HRTEM, as the boundary between disordered fluorite and pyrochlore matrix is less distinct. However, the C 60 irradiation shows a clearly resolved ion track with completely crystalline, disordered, defect-fluorite structure around an amorphous core. Based on the distinct boundaries of the track morphology, inelastic thermal-spike calculations were used to describe the track size and extract critical energy densities for the interpretation of the complex core–shell morphologies for the different pyrochlore compositions. More... »

PAGES

2456-2466

Identifiers

URI

http://scigraph.springernature.com/pub.10.1557/jmr.2015.230

DOI

http://dx.doi.org/10.1557/jmr.2015.230

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1022767364


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