Chemical Vapor Deposition of Vertically Aligned Carbon Nanotube Arrays: Critical Effects of Oxide Buffer Layers View Full Text


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Article Info

DATE

2019-12

AUTHORS

Haohao Li, Guangjie Yuan, Bo Shan, Xiaoxin Zhang, Hongping Ma, Yingzhong Tian, Hongliang Lu, Johan Liu

ABSTRACT

Vertically aligned carbon nanotubes (VACNTs) were synthesized on different oxide buffer layers using chemical vapor deposition (CVD). The growth of the VACNTs was mainly determined by three factors: the Ostwald ripening of catalyst nanoparticles, subsurface diffusion of Fe, and their activation energy for nucleation and initial growth. The surface roughness of buffer layers largely influenced the diameter and density of catalyst nanoparticles after annealing, which apparently affected the lifetime of the nanoparticles and the thickness of the prepared VACNTs. In addition, the growth of the VACNTs was also affected by the deposition temperature, and the lifetime of the catalyst nanoparticles apparently decreased when the deposition temperature was greater than 600 °C due to their serious Ostwald ripening. Furthermore, in addition to the number of catalyst nanoparticles, the density of the VACNTs was also largely dependent on their activation energy for nucleation and initial growth. More... »

PAGES

106

Identifiers

URI

http://scigraph.springernature.com/pub.10.1186/s11671-019-2938-6

DOI

http://dx.doi.org/10.1186/s11671-019-2938-6

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1112926575

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30900108


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