A Facile Way to Fabricate High-Performance Solution-Processed n-MoS2/p-MoS2 Bilayer Photodetectors View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2015-12

AUTHORS

Jian Ye, Xueliang Li, Jianjun Zhao, Xuelan Mei, Qian Li

ABSTRACT

Two-dimensional (2D) material has many advantages including high carrier mobilities and conductivity, high optical transparency, excellent mechanical flexibility, and chemical stability, which made 2D material an ideal material for various optoelectronic devices. Here, we developed a facile method of preparing MoS2 nanosheets followed by a facile liquid exfoliation method via ethyl cellulose-assisted doping and utilizing a plasma-induced p-doping approach to generate t effectively the partially oxided MoS2 (p-MoS2) nanosheets from the pristine n-type nanosheets. Moreover, an n-p junction type MoS2 photodetector device with the built-in potentials to separate the photogenerated charges is able to significantly improved visible light response. We have fabricated photodetector devices consisting of a vertically stacked indium tin oxide (ITO)/pristine n-type MoS2 nanosheets/p-MoS2/Ag structure, which exhibit reasonably good performance illumination, as well as high current values in the range of visible wavelength from 350 to 600 nm. We believe that this work provides important scientific insights for photoelectric response properties of emerging atomically layered 2D materials for photovoltaic and other optoelectronic applications. More... »

PAGES

454

Identifiers

URI

http://scigraph.springernature.com/pub.10.1186/s11671-015-1161-3

DOI

http://dx.doi.org/10.1186/s11671-015-1161-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1016793656

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26608537


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53 schema:description Two-dimensional (2D) material has many advantages including high carrier mobilities and conductivity, high optical transparency, excellent mechanical flexibility, and chemical stability, which made 2D material an ideal material for various optoelectronic devices. Here, we developed a facile method of preparing MoS2 nanosheets followed by a facile liquid exfoliation method via ethyl cellulose-assisted doping and utilizing a plasma-induced p-doping approach to generate t effectively the partially oxided MoS2 (p-MoS2) nanosheets from the pristine n-type nanosheets. Moreover, an n-p junction type MoS2 photodetector device with the built-in potentials to separate the photogenerated charges is able to significantly improved visible light response. We have fabricated photodetector devices consisting of a vertically stacked indium tin oxide (ITO)/pristine n-type MoS2 nanosheets/p-MoS2/Ag structure, which exhibit reasonably good performance illumination, as well as high current values in the range of visible wavelength from 350 to 600 nm. We believe that this work provides important scientific insights for photoelectric response properties of emerging atomically layered 2D materials for photovoltaic and other optoelectronic applications.
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