The Daoud and Cotton blob model and the interaction of star-shaped polymers View Full Text


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Article Info

DATE

2018-07

AUTHORS

Albert Johner, Nam-Kyung Lee

ABSTRACT

Since it was first proposed in 1982, the Daoud and Cotton (DC) model for star-shaped polymers was intensively used also for self-assembled copolymers and small colloids grafted with long polymers. We try to clarify the position of the DC model and focus on the star partition function which plays a central role in self-assembly and gives access to the star-star interaction. While the predicted star-star interaction agrees with scattering data by Likos et al. (Phys. Rev. Lett. 80, 4450 (1998)), an extensive simulation by Hsu et al. (Macromolecules, 37, 4658 (2004)) does not recover the prediction for the partition function. We try to reconcile this seemingly conflicting results. We discuss star-star interactions, star free energy in θ -solvents, mixing of A/B branches in copolymer stars, within or beyond the Daoud and Cotton blob model. More... »

PAGES

88

References to SciGraph publications

  • 2000-08. Triplet interactions in star polymer solutions in THE EUROPEAN PHYSICAL JOURNAL E
  • 1989-02. Statistical mechanics of polymer networks of any topology in JOURNAL OF STATISTICAL PHYSICS
  • 1998-06. Scattering from solutions of star polymers in THE EUROPEAN PHYSICAL JOURNAL B
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    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/30039228


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