Depletion of ideal polymer chains near a spherical colloid particle beyond the Dirichlet boundary conditions View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2010-02

AUTHORS

I. Erukhimovich, A. Johner, J. F. Joanny

ABSTRACT

We reconsider the depletion interaction of an ideal polymer chain, characterized by the gyration radius R(G) and bond length a , and an impenetrable spherical colloid particle of radius R . Forbidding the polymer-colloid penetration explicitly (by the use of Mayer functions) without any other requirement we derive and solve analytically an integral equation for the chain partition function of a long ideal polymer chain for the spherical geometry. We find that the correction to the solution of the Dirichlet problem depends on the ratios R/R (G) and R/a . The correction vanishes for the continuous chain model (i.e. in the limit R/R (G) --> 0 and R/a --> infinity but stays finite (even for an infinite chain) for the discrete chain model. The correction can become substantial in the case of nano-colloids (the so-called protein limit). More... »

PAGES

115-124

Identifiers

URI

http://scigraph.springernature.com/pub.10.1140/epje/i2010-10568-4

DOI

http://dx.doi.org/10.1140/epje/i2010-10568-4

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1018652973

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/20174851


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