Formation and photofragmentation properties of isolated aromatic amino acid-silver cluster hybrids View Full Text


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Article Info

DATE

2009-04

AUTHORS

T. Tabarin, R. Antoine, M. Broyer, P. Dugourd

ABSTRACT

The formation of isolated [ (Trp-2H)+Ag9] + and [ (Tyr-2H)+Ag9] + amino-acid-Ag9 hybrids is reported. The photofragmentation yields of the aromatic amino acid-silver cluster hybrids, as well as those of the protonated tryptophan and tyrosine molecules ([Trp+H]+ and [Tyr+H]+) have been recorded. The fragmentation yields of the complexes are higher than the yields for [Trp+H]+and [Tyr+H]+ and present an extension of the fragmentation on the red side of the spectrum. The photofragmentation spectrum of [ Trp+Ag9] + was recently reported [Mitric et al., J. Chem. Phys. 127, 134301 (2007)]. While the optical spectra of substituted [ (Trp-2H)+Ag9] + and non-substituted [ Trp+Ag9] + complexes are very similar, a strong modification of the fragmentation channels between the two complexes is observed. The fragmentation channels are sensitive to the type of bonding in aromatic amino acid-silver cluster hybrids and can be used as fingerprints of structures. More... »

PAGES

191-194

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URI

http://scigraph.springernature.com/pub.10.1140/epjd/e2008-00272-2

DOI

http://dx.doi.org/10.1140/epjd/e2008-00272-2

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https://app.dimensions.ai/details/publication/pub.1034309914


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