Effects of confinement on the electron and lattice dynamics in metal nanoparticles View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2005-07

AUTHORS

J. Lermé, G. Celep, M. Broyer, E. Cottancin, M. Pellarin, A. Arbouet, D. Christofilos, C. Guillon, P. Langot, N. Del Fatti, F. Vallée

ABSTRACT

Effects of confinement on the electron-electron (e-e) and electron-phonon (e-ph) thermalization dynamics in noble metal clusters are calculated using simple approaches. The model predictions are compared with femtosecond pump-probe measurements which display an acceleration of the e-e and e-ph relaxation dynamics. The size-effects on the e-e relaxation dynamics are consistent with a model involving the surface-induced reduction of the screening efficiency of the Coulomb e-e interaction. With regard to the e-ph relaxation dynamics, this model yields too large time constants, pointing out deficiencies of the standard modelling of the e-ph energy exchanges in bulk metals. Analysis of these deficiencies shows that the bare e-ion interaction has to be involved in the transition matrix element describing the non-adiabatic e-ph energy exchanges. More... »

PAGES

199-204

Identifiers

URI

http://scigraph.springernature.com/pub.10.1140/epjd/e2005-00107-8

DOI

http://dx.doi.org/10.1140/epjd/e2005-00107-8

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1009491503


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