Binuclear complexes of copper(II) with 1′-phthalazinylhydrazones of substituted salicylic aldehydes: Physico-chemical study and quantum-chemical simulation View Full Text


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Article Info

DATE

2014-10

AUTHORS

S. I. Levchenkov, L. D. Popov, I. N. Shcherbakov, V. G. Vlasenko, A. A. Tsaturyan, S. S. Beloborodov, A. M. Ionov, V. A. Kogan

ABSTRACT

Binuclear complexes of copper(II) with 1′-phthalazinylhydrazones of substituted salicylic aldehydes have been prepared and studied. Antiferromagnetic exchange interaction between copper(II) ions has been revealed in all the complexes. Taking advantage of quantum-chemical simulation, we have investigated the influence of the complexes structural isomerism on the character of the exchange interaction between the paramagnetic centers. X-ray absorbance spectroscopy afforded the structural parameters of coordination spheres of copper(II) ions; it has been demonstrated that dimerization occurred via the nitrogen atoms of phthalazine fragments. More... »

PAGES

1970-1978

References to SciGraph publications

  • 2013-09. Tautomerism of substituted salicylaldehyde and 2-diphenylphosphinebenzaldehyde 1′-phthalazinylhydrazones: X-ray crystallography and quantum chemical modeling in JOURNAL OF STRUCTURAL CHEMISTRY
  • 2011-07. Crystal structure and magnetic properties of the binuclear copper(II) complex based on 1,3-diaminopropan-2-ol N,N′-bis(3-formyl-5-tert-butylsalicylidene) in RUSSIAN JOURNAL OF COORDINATION CHEMISTRY
  • 2012-03. X-ray absorption spectroscopic and magneto-chemical analysis of the atomic structure of copper(II) complexes with diacetyl monoxime 1′-phthalazinyl hydrazone in JOURNAL OF STRUCTURAL CHEMISTRY
  • 2009-04. Specificity of complex formation of benzoin (phthalazin-1-yl)hydrazone with copper(II) and nickel(II): Physicochemical study and quantum-chemical simulation in RUSSIAN JOURNAL OF GENERAL CHEMISTRY
  • 2009-12. 1-Hydrazinophthalazine based hydrazones and their transition metal complexes: Structure and biological activity in RUSSIAN JOURNAL OF GENERAL CHEMISTRY
  • 2009-08. Influence of structural factors on the magnetic properties of the binuclear copper complexes with salicylaldehyde hydrazone and bis(hydrazone)-2,6-diformylphenol: Quantum-chemical calculations in RUSSIAN JOURNAL OF COORDINATION CHEMISTRY
  • 1992-09. Fluorimetric determination of trace amounts of aluminium and gallium with salicylaldehyde-1-phthalazinohydrazone in MICROCHIMICA ACTA
  • 2010-03. 1′-Phthalazine hydrazone of diacetyl monooxime and its complexes with transition metals: Physicochemical and theoretical study in RUSSIAN JOURNAL OF GENERAL CHEMISTRY
  • 2003-05. Mono- and Binuclear Copper(II) Metal Chelates with 3,5-Di(tert-butyl)salicylaldehyde Acylhydrazones in RUSSIAN JOURNAL OF COORDINATION CHEMISTRY
  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1134/s1070363214100193

    DOI

    http://dx.doi.org/10.1134/s1070363214100193

    DIMENSIONS

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    36 schema:description Binuclear complexes of copper(II) with 1′-phthalazinylhydrazones of substituted salicylic aldehydes have been prepared and studied. Antiferromagnetic exchange interaction between copper(II) ions has been revealed in all the complexes. Taking advantage of quantum-chemical simulation, we have investigated the influence of the complexes structural isomerism on the character of the exchange interaction between the paramagnetic centers. X-ray absorbance spectroscopy afforded the structural parameters of coordination spheres of copper(II) ions; it has been demonstrated that dimerization occurred via the nitrogen atoms of phthalazine fragments.
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