Radionuclides in Irradiated Graphite of Uranium–Graphite Reactors: Decontamination of Sleeves Using Liquid Reagents View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2018-09

AUTHORS

A. G. Volkova, E. V. Zakharova, A. O. Pavlyuk, A. A. Shiryaev

ABSTRACT

To examine the possibility of disposal of irradiated graphite in ground near-surface repositories, the concentration and spatial distribution of radionuclides in the volume of irradiated graphite sleeves of industrial uranium–graphite reactors was studied, and the efficiency of decontamination using liquid reagent treatment methods was evaluated. The radionuclide distribution in the graphite volume is extremely heterogeneous on the 10–100 μm scale. The degree of decontamination using solutions with high acid concentrations and fluoride ions added does not exceed 16–25% for 14C and 15–19% for 36Cl. Under these treatment conditions, no structural changes occur in graphite, and 14С bound with the graphite surface via sorption is removed. Significant differences in the efficiency of the reagent decontamination of irradiated graphite from various producers were revealed. More... »

PAGES

558-562

References to SciGraph publications

Journal

TITLE

Radiochemistry

ISSUE

5

VOLUME

60

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s1066362218050144

DOI

http://dx.doi.org/10.1134/s1066362218050144

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1110131776


Indexing Status Check whether this publication has been indexed by Scopus and Web Of Science using the SN Indexing Status Tool
Incoming Citations Browse incoming citations for this publication using opencitations.net

JSON-LD is the canonical representation for SciGraph data.

TIP: You can open this SciGraph record using an external JSON-LD service: JSON-LD Playground Google SDTT

[
  {
    "@context": "https://springernature.github.io/scigraph/jsonld/sgcontext.json", 
    "about": [
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0912", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Materials Engineering", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/09", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Engineering", 
        "type": "DefinedTerm"
      }
    ], 
    "author": [
      {
        "affiliation": {
          "alternateName": "Russian Academy of Sciences", 
          "id": "https://www.grid.ac/institutes/grid.4886.2", 
          "name": [
            "Frumkin Institute of Physical Chemistry and Electrochemistry, Russian Academy of Sciences, Leninskii pr. 31, korp. 4, 119071, Moscow, Russia"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Volkova", 
        "givenName": "A. G.", 
        "id": "sg:person.011140372520.99", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.011140372520.99"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Russian Academy of Sciences", 
          "id": "https://www.grid.ac/institutes/grid.4886.2", 
          "name": [
            "Frumkin Institute of Physical Chemistry and Electrochemistry, Russian Academy of Sciences, Leninskii pr. 31, korp. 4, 119071, Moscow, Russia"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Zakharova", 
        "givenName": "E. V.", 
        "id": "sg:person.010343012120.48", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010343012120.48"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "name": [
            "Experimental and Demonstration Center for Decommissioning of Uranium\u2013Graphite Reactors, P.O. Box 654, 636000, Seversk, Tomsk oblast, Russia"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Pavlyuk", 
        "givenName": "A. O.", 
        "id": "sg:person.015312344017.73", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.015312344017.73"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Russian Academy of Sciences", 
          "id": "https://www.grid.ac/institutes/grid.4886.2", 
          "name": [
            "Frumkin Institute of Physical Chemistry and Electrochemistry, Russian Academy of Sciences, Leninskii pr. 31, korp. 4, 119071, Moscow, Russia"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Shiryaev", 
        "givenName": "A. A.", 
        "type": "Person"
      }
    ], 
    "citation": [
      {
        "id": "sg:pub.10.1007/s10512-012-9525-6", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1000265900", 
          "https://doi.org/10.1007/s10512-012-9525-6"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1007/s10512-011-9449-6", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1013471377", 
          "https://doi.org/10.1007/s10512-011-9449-6"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1134/s1061934815030107", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1013560299", 
          "https://doi.org/10.1134/s1061934815030107"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1007/bf00761431", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1020146299", 
          "https://doi.org/10.1007/bf00761431"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1007/bf00761431", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1020146299", 
          "https://doi.org/10.1007/bf00761431"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1023/a:1023629020300", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1021397927", 
          "https://doi.org/10.1023/a:1023629020300"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1007/s10512-014-9910-4", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1030075281", 
          "https://doi.org/10.1007/s10512-014-9910-4"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "https://doi.org/10.1016/j.nucengdes.2008.02.010", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1032083750"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1023/a:1011351525683", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1036800096", 
          "https://doi.org/10.1023/a:1011351525683"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "https://doi.org/10.1016/j.jnucmat.2013.02.027", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1051211392"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "https://doi.org/10.1524/ract.2010.1767", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1067647841"
        ], 
        "type": "CreativeWork"
      }
    ], 
    "datePublished": "2018-09", 
    "datePublishedReg": "2018-09-01", 
    "description": "To examine the possibility of disposal of irradiated graphite in ground near-surface repositories, the concentration and spatial distribution of radionuclides in the volume of irradiated graphite sleeves of industrial uranium\u2013graphite reactors was studied, and the efficiency of decontamination using liquid reagent treatment methods was evaluated. The radionuclide distribution in the graphite volume is extremely heterogeneous on the 10\u2013100 \u03bcm scale. The degree of decontamination using solutions with high acid concentrations and fluoride ions added does not exceed 16\u201325% for 14C and 15\u201319% for 36Cl. Under these treatment conditions, no structural changes occur in graphite, and 14\u0421 bound with the graphite surface via sorption is removed. Significant differences in the efficiency of the reagent decontamination of irradiated graphite from various producers were revealed.", 
    "genre": "research_article", 
    "id": "sg:pub.10.1134/s1066362218050144", 
    "inLanguage": [
      "en"
    ], 
    "isAccessibleForFree": false, 
    "isPartOf": [
      {
        "id": "sg:journal.1345524", 
        "issn": [
          "1066-3622", 
          "1608-3288"
        ], 
        "name": "Radiochemistry", 
        "type": "Periodical"
      }, 
      {
        "issueNumber": "5", 
        "type": "PublicationIssue"
      }, 
      {
        "type": "PublicationVolume", 
        "volumeNumber": "60"
      }
    ], 
    "name": "Radionuclides in Irradiated Graphite of Uranium\u2013Graphite Reactors: Decontamination of Sleeves Using Liquid Reagents", 
    "pagination": "558-562", 
    "productId": [
      {
        "name": "readcube_id", 
        "type": "PropertyValue", 
        "value": [
          "e38a710f72c9fb45352e92b492c297cb0325f32794fdb2833a04461bbc5b8ba3"
        ]
      }, 
      {
        "name": "doi", 
        "type": "PropertyValue", 
        "value": [
          "10.1134/s1066362218050144"
        ]
      }, 
      {
        "name": "dimensions_id", 
        "type": "PropertyValue", 
        "value": [
          "pub.1110131776"
        ]
      }
    ], 
    "sameAs": [
      "https://doi.org/10.1134/s1066362218050144", 
      "https://app.dimensions.ai/details/publication/pub.1110131776"
    ], 
    "sdDataset": "articles", 
    "sdDatePublished": "2019-04-11T08:11", 
    "sdLicense": "https://scigraph.springernature.com/explorer/license/", 
    "sdPublisher": {
      "name": "Springer Nature - SN SciGraph project", 
      "type": "Organization"
    }, 
    "sdSource": "s3://com-uberresearch-data-dimensions-target-20181106-alternative/cleanup/v134/2549eaecd7973599484d7c17b260dba0a4ecb94b/merge/v9/a6c9fde33151104705d4d7ff012ea9563521a3ce/jats-lookup/v90/0000000270_0000000270/records_9665_00000000.jsonl", 
    "type": "ScholarlyArticle", 
    "url": "https://link.springer.com/10.1134%2FS1066362218050144"
  }
]
 

Download the RDF metadata as:  json-ld nt turtle xml License info

HOW TO GET THIS DATA PROGRAMMATICALLY:

JSON-LD is a popular format for linked data which is fully compatible with JSON.

curl -H 'Accept: application/ld+json' 'https://scigraph.springernature.com/pub.10.1134/s1066362218050144'

N-Triples is a line-based linked data format ideal for batch operations.

curl -H 'Accept: application/n-triples' 'https://scigraph.springernature.com/pub.10.1134/s1066362218050144'

Turtle is a human-readable linked data format.

curl -H 'Accept: text/turtle' 'https://scigraph.springernature.com/pub.10.1134/s1066362218050144'

RDF/XML is a standard XML format for linked data.

curl -H 'Accept: application/rdf+xml' 'https://scigraph.springernature.com/pub.10.1134/s1066362218050144'


 

This table displays all metadata directly associated to this object as RDF triples.

120 TRIPLES      21 PREDICATES      37 URIs      19 LITERALS      7 BLANK NODES

Subject Predicate Object
1 sg:pub.10.1134/s1066362218050144 schema:about anzsrc-for:09
2 anzsrc-for:0912
3 schema:author N0bd259f92d824b5cb0019b148f3bdcbe
4 schema:citation sg:pub.10.1007/bf00761431
5 sg:pub.10.1007/s10512-011-9449-6
6 sg:pub.10.1007/s10512-012-9525-6
7 sg:pub.10.1007/s10512-014-9910-4
8 sg:pub.10.1023/a:1011351525683
9 sg:pub.10.1023/a:1023629020300
10 sg:pub.10.1134/s1061934815030107
11 https://doi.org/10.1016/j.jnucmat.2013.02.027
12 https://doi.org/10.1016/j.nucengdes.2008.02.010
13 https://doi.org/10.1524/ract.2010.1767
14 schema:datePublished 2018-09
15 schema:datePublishedReg 2018-09-01
16 schema:description To examine the possibility of disposal of irradiated graphite in ground near-surface repositories, the concentration and spatial distribution of radionuclides in the volume of irradiated graphite sleeves of industrial uranium–graphite reactors was studied, and the efficiency of decontamination using liquid reagent treatment methods was evaluated. The radionuclide distribution in the graphite volume is extremely heterogeneous on the 10–100 μm scale. The degree of decontamination using solutions with high acid concentrations and fluoride ions added does not exceed 16–25% for 14C and 15–19% for 36Cl. Under these treatment conditions, no structural changes occur in graphite, and 14С bound with the graphite surface via sorption is removed. Significant differences in the efficiency of the reagent decontamination of irradiated graphite from various producers were revealed.
17 schema:genre research_article
18 schema:inLanguage en
19 schema:isAccessibleForFree false
20 schema:isPartOf N3959ab366cd34d749d9476675ff30aec
21 Nbb74070a0f95411ba9c793b5c035c930
22 sg:journal.1345524
23 schema:name Radionuclides in Irradiated Graphite of Uranium–Graphite Reactors: Decontamination of Sleeves Using Liquid Reagents
24 schema:pagination 558-562
25 schema:productId N3b0a6dd68c114aba852af7329d3330d0
26 N858fbc9af5e04572bde334056ad4d640
27 Nc0eeecb804cc4512b33bb40e0c4fd96d
28 schema:sameAs https://app.dimensions.ai/details/publication/pub.1110131776
29 https://doi.org/10.1134/s1066362218050144
30 schema:sdDatePublished 2019-04-11T08:11
31 schema:sdLicense https://scigraph.springernature.com/explorer/license/
32 schema:sdPublisher N92497a2685c643ae8fee67358d6eaa54
33 schema:url https://link.springer.com/10.1134%2FS1066362218050144
34 sgo:license sg:explorer/license/
35 sgo:sdDataset articles
36 rdf:type schema:ScholarlyArticle
37 N084bc5ba12da43779f26aa085049618f schema:affiliation https://www.grid.ac/institutes/grid.4886.2
38 schema:familyName Shiryaev
39 schema:givenName A. A.
40 rdf:type schema:Person
41 N0bd259f92d824b5cb0019b148f3bdcbe rdf:first sg:person.011140372520.99
42 rdf:rest N3891020bcd8e48b5823fa8d78cf6aa20
43 N3891020bcd8e48b5823fa8d78cf6aa20 rdf:first sg:person.010343012120.48
44 rdf:rest N6a1500d1af314abfa49b508c3f7da38b
45 N3959ab366cd34d749d9476675ff30aec schema:volumeNumber 60
46 rdf:type schema:PublicationVolume
47 N3b0a6dd68c114aba852af7329d3330d0 schema:name dimensions_id
48 schema:value pub.1110131776
49 rdf:type schema:PropertyValue
50 N6a1500d1af314abfa49b508c3f7da38b rdf:first sg:person.015312344017.73
51 rdf:rest N70d86f42ac7e434e9db889ceb6bc0af7
52 N70d86f42ac7e434e9db889ceb6bc0af7 rdf:first N084bc5ba12da43779f26aa085049618f
53 rdf:rest rdf:nil
54 N858fbc9af5e04572bde334056ad4d640 schema:name doi
55 schema:value 10.1134/s1066362218050144
56 rdf:type schema:PropertyValue
57 N92497a2685c643ae8fee67358d6eaa54 schema:name Springer Nature - SN SciGraph project
58 rdf:type schema:Organization
59 N957e3332da4045f0807b72a061159f5d schema:name Experimental and Demonstration Center for Decommissioning of Uranium–Graphite Reactors, P.O. Box 654, 636000, Seversk, Tomsk oblast, Russia
60 rdf:type schema:Organization
61 Nbb74070a0f95411ba9c793b5c035c930 schema:issueNumber 5
62 rdf:type schema:PublicationIssue
63 Nc0eeecb804cc4512b33bb40e0c4fd96d schema:name readcube_id
64 schema:value e38a710f72c9fb45352e92b492c297cb0325f32794fdb2833a04461bbc5b8ba3
65 rdf:type schema:PropertyValue
66 anzsrc-for:09 schema:inDefinedTermSet anzsrc-for:
67 schema:name Engineering
68 rdf:type schema:DefinedTerm
69 anzsrc-for:0912 schema:inDefinedTermSet anzsrc-for:
70 schema:name Materials Engineering
71 rdf:type schema:DefinedTerm
72 sg:journal.1345524 schema:issn 1066-3622
73 1608-3288
74 schema:name Radiochemistry
75 rdf:type schema:Periodical
76 sg:person.010343012120.48 schema:affiliation https://www.grid.ac/institutes/grid.4886.2
77 schema:familyName Zakharova
78 schema:givenName E. V.
79 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010343012120.48
80 rdf:type schema:Person
81 sg:person.011140372520.99 schema:affiliation https://www.grid.ac/institutes/grid.4886.2
82 schema:familyName Volkova
83 schema:givenName A. G.
84 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.011140372520.99
85 rdf:type schema:Person
86 sg:person.015312344017.73 schema:affiliation N957e3332da4045f0807b72a061159f5d
87 schema:familyName Pavlyuk
88 schema:givenName A. O.
89 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.015312344017.73
90 rdf:type schema:Person
91 sg:pub.10.1007/bf00761431 schema:sameAs https://app.dimensions.ai/details/publication/pub.1020146299
92 https://doi.org/10.1007/bf00761431
93 rdf:type schema:CreativeWork
94 sg:pub.10.1007/s10512-011-9449-6 schema:sameAs https://app.dimensions.ai/details/publication/pub.1013471377
95 https://doi.org/10.1007/s10512-011-9449-6
96 rdf:type schema:CreativeWork
97 sg:pub.10.1007/s10512-012-9525-6 schema:sameAs https://app.dimensions.ai/details/publication/pub.1000265900
98 https://doi.org/10.1007/s10512-012-9525-6
99 rdf:type schema:CreativeWork
100 sg:pub.10.1007/s10512-014-9910-4 schema:sameAs https://app.dimensions.ai/details/publication/pub.1030075281
101 https://doi.org/10.1007/s10512-014-9910-4
102 rdf:type schema:CreativeWork
103 sg:pub.10.1023/a:1011351525683 schema:sameAs https://app.dimensions.ai/details/publication/pub.1036800096
104 https://doi.org/10.1023/a:1011351525683
105 rdf:type schema:CreativeWork
106 sg:pub.10.1023/a:1023629020300 schema:sameAs https://app.dimensions.ai/details/publication/pub.1021397927
107 https://doi.org/10.1023/a:1023629020300
108 rdf:type schema:CreativeWork
109 sg:pub.10.1134/s1061934815030107 schema:sameAs https://app.dimensions.ai/details/publication/pub.1013560299
110 https://doi.org/10.1134/s1061934815030107
111 rdf:type schema:CreativeWork
112 https://doi.org/10.1016/j.jnucmat.2013.02.027 schema:sameAs https://app.dimensions.ai/details/publication/pub.1051211392
113 rdf:type schema:CreativeWork
114 https://doi.org/10.1016/j.nucengdes.2008.02.010 schema:sameAs https://app.dimensions.ai/details/publication/pub.1032083750
115 rdf:type schema:CreativeWork
116 https://doi.org/10.1524/ract.2010.1767 schema:sameAs https://app.dimensions.ai/details/publication/pub.1067647841
117 rdf:type schema:CreativeWork
118 https://www.grid.ac/institutes/grid.4886.2 schema:alternateName Russian Academy of Sciences
119 schema:name Frumkin Institute of Physical Chemistry and Electrochemistry, Russian Academy of Sciences, Leninskii pr. 31, korp. 4, 119071, Moscow, Russia
120 rdf:type schema:Organization
 




Preview window. Press ESC to close (or click here)


...