Emission Kinetics of Surface (Bi)Excitons in ZnO Thin Films View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2019-03

AUTHORS

I. Kh. Akopyan, M. E. Labzovskaya, B. V. Novikov, V. G. Talalaev, J. W. Tomm, J. Schilling

ABSTRACT

The kinetics of near-edge photoluminescence (PL) in ZnO nanofilms prepared by the atomic layer deposition has been investigated. It is established that the kinetics of near-edge PL in 4-nm films is determined to a great extent by surface 2D-exciton (SX) and biexciton (SXX) complexes. The contribution from surface biexcitons is estimated based on a photostimulated change in the surface potential in ZnO films with different thicknesses. Ultrafast dynamics of surface biexcitons in thin films are revealed. It is shown that biexcitons localized near the surface have the shortest radiative lifetime (less than 100 ps) among all bound exciton complexes, which is explained by the large oscillator strength. More... »

PAGES

402-407

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s1063783419030041

DOI

http://dx.doi.org/10.1134/s1063783419030041

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1113627074


Indexing Status Check whether this publication has been indexed by Scopus and Web Of Science using the SN Indexing Status Tool
Incoming Citations Browse incoming citations for this publication using opencitations.net

JSON-LD is the canonical representation for SciGraph data.

TIP: You can open this SciGraph record using an external JSON-LD service: JSON-LD Playground Google SDTT

[
  {
    "@context": "https://springernature.github.io/scigraph/jsonld/sgcontext.json", 
    "about": [
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/02", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Physical Sciences", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0203", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Classical Physics", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0204", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Condensed Matter Physics", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0206", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Quantum Physics", 
        "type": "DefinedTerm"
      }
    ], 
    "author": [
      {
        "affiliation": {
          "alternateName": "St. Petersburg State University, 199034, St. Petersburg, Russia", 
          "id": "http://www.grid.ac/institutes/grid.15447.33", 
          "name": [
            "St. Petersburg State University, 199034, St. Petersburg, Russia"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Akopyan", 
        "givenName": "I. Kh.", 
        "id": "sg:person.012314723253.70", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.012314723253.70"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "St. Petersburg State University, 199034, St. Petersburg, Russia", 
          "id": "http://www.grid.ac/institutes/grid.15447.33", 
          "name": [
            "St. Petersburg State University, 199034, St. Petersburg, Russia"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Labzovskaya", 
        "givenName": "M. E.", 
        "id": "sg:person.013444462541.44", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.013444462541.44"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "St. Petersburg State University, 199034, St. Petersburg, Russia", 
          "id": "http://www.grid.ac/institutes/grid.15447.33", 
          "name": [
            "St. Petersburg State University, 199034, St. Petersburg, Russia"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Novikov", 
        "givenName": "B. V.", 
        "id": "sg:person.014034276053.56", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.014034276053.56"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Martin-Luther University, Centre for Innovation Competence SiLi-nano, Halle, Germany", 
          "id": "http://www.grid.ac/institutes/grid.9018.0", 
          "name": [
            "Martin-Luther University, Centre for Innovation Competence SiLi-nano, Halle, Germany"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Talalaev", 
        "givenName": "V. G.", 
        "id": "sg:person.0615207126.40", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0615207126.40"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Berlin, Germany", 
          "id": "http://www.grid.ac/institutes/grid.419569.6", 
          "name": [
            "Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Berlin, Germany"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Tomm", 
        "givenName": "J. W.", 
        "id": "sg:person.013312125473.62", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.013312125473.62"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Martin-Luther University, Centre for Innovation Competence SiLi-nano, Halle, Germany", 
          "id": "http://www.grid.ac/institutes/grid.9018.0", 
          "name": [
            "Martin-Luther University, Centre for Innovation Competence SiLi-nano, Halle, Germany"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Schilling", 
        "givenName": "J.", 
        "id": "sg:person.014037377704.20", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.014037377704.20"
        ], 
        "type": "Person"
      }
    ], 
    "citation": [
      {
        "id": "sg:pub.10.1134/s1063783418020026", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1101289295", 
          "https://doi.org/10.1134/s1063783418020026"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1134/s1063783416090031", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1019743702", 
          "https://doi.org/10.1134/s1063783416090031"
        ], 
        "type": "CreativeWork"
      }, 
      {
        "id": "sg:pub.10.1007/978-3-642-10577-7", 
        "sameAs": [
          "https://app.dimensions.ai/details/publication/pub.1038674452", 
          "https://doi.org/10.1007/978-3-642-10577-7"
        ], 
        "type": "CreativeWork"
      }
    ], 
    "datePublished": "2019-03", 
    "datePublishedReg": "2019-03-01", 
    "description": "The kinetics of near-edge photoluminescence (PL) in ZnO nanofilms prepared by the atomic layer deposition has been investigated. It is established that the kinetics of near-edge PL in 4-nm films is determined to a great extent by surface 2D-exciton (SX) and biexciton (SXX) complexes. The contribution from surface biexcitons is estimated based on a photostimulated change in the surface potential in ZnO films with different thicknesses. Ultrafast dynamics of surface biexcitons in thin films are revealed. It is shown that biexcitons localized near the surface have the shortest radiative lifetime (less than 100 ps) among all bound exciton complexes, which is explained by the large oscillator strength.", 
    "genre": "article", 
    "id": "sg:pub.10.1134/s1063783419030041", 
    "inLanguage": "en", 
    "isAccessibleForFree": false, 
    "isFundedItemOf": [
      {
        "id": "sg:grant.7595746", 
        "type": "MonetaryGrant"
      }
    ], 
    "isPartOf": [
      {
        "id": "sg:journal.1136591", 
        "issn": [
          "0367-3294", 
          "1063-7834"
        ], 
        "name": "Physics of the Solid State", 
        "publisher": "Pleiades Publishing", 
        "type": "Periodical"
      }, 
      {
        "issueNumber": "3", 
        "type": "PublicationIssue"
      }, 
      {
        "type": "PublicationVolume", 
        "volumeNumber": "61"
      }
    ], 
    "keywords": [
      "thin films", 
      "large oscillator strength", 
      "short radiative lifetime", 
      "ZnO thin films", 
      "ultrafast dynamics", 
      "biexciton complexes", 
      "exciton complexes", 
      "radiative lifetimes", 
      "oscillator strengths", 
      "atomic layer deposition", 
      "ZnO films", 
      "biexciton", 
      "ZnO nanofilms", 
      "photoluminescence", 
      "emission kinetics", 
      "photostimulated changes", 
      "layer deposition", 
      "surface potential", 
      "films", 
      "different thicknesses", 
      "complexes", 
      "kinetics", 
      "surface", 
      "nanofilms", 
      "lifetime", 
      "deposition", 
      "thickness", 
      "dynamics", 
      "strength", 
      "potential", 
      "greater extent", 
      "contribution", 
      "extent", 
      "changes"
    ], 
    "name": "Emission Kinetics of Surface (Bi)Excitons in ZnO Thin Films", 
    "pagination": "402-407", 
    "productId": [
      {
        "name": "dimensions_id", 
        "type": "PropertyValue", 
        "value": [
          "pub.1113627074"
        ]
      }, 
      {
        "name": "doi", 
        "type": "PropertyValue", 
        "value": [
          "10.1134/s1063783419030041"
        ]
      }
    ], 
    "sameAs": [
      "https://doi.org/10.1134/s1063783419030041", 
      "https://app.dimensions.ai/details/publication/pub.1113627074"
    ], 
    "sdDataset": "articles", 
    "sdDatePublished": "2022-05-20T07:35", 
    "sdLicense": "https://scigraph.springernature.com/explorer/license/", 
    "sdPublisher": {
      "name": "Springer Nature - SN SciGraph project", 
      "type": "Organization"
    }, 
    "sdSource": "s3://com-springernature-scigraph/baseset/20220519/entities/gbq_results/article/article_812.jsonl", 
    "type": "ScholarlyArticle", 
    "url": "https://doi.org/10.1134/s1063783419030041"
  }
]
 

Download the RDF metadata as:  json-ld nt turtle xml License info

HOW TO GET THIS DATA PROGRAMMATICALLY:

JSON-LD is a popular format for linked data which is fully compatible with JSON.

curl -H 'Accept: application/ld+json' 'https://scigraph.springernature.com/pub.10.1134/s1063783419030041'

N-Triples is a line-based linked data format ideal for batch operations.

curl -H 'Accept: application/n-triples' 'https://scigraph.springernature.com/pub.10.1134/s1063783419030041'

Turtle is a human-readable linked data format.

curl -H 'Accept: text/turtle' 'https://scigraph.springernature.com/pub.10.1134/s1063783419030041'

RDF/XML is a standard XML format for linked data.

curl -H 'Accept: application/rdf+xml' 'https://scigraph.springernature.com/pub.10.1134/s1063783419030041'


 

This table displays all metadata directly associated to this object as RDF triples.

155 TRIPLES      22 PREDICATES      65 URIs      52 LITERALS      6 BLANK NODES

Subject Predicate Object
1 sg:pub.10.1134/s1063783419030041 schema:about anzsrc-for:02
2 anzsrc-for:0203
3 anzsrc-for:0204
4 anzsrc-for:0206
5 schema:author N57fd6f520a1644be84ed1dba7bc0312d
6 schema:citation sg:pub.10.1007/978-3-642-10577-7
7 sg:pub.10.1134/s1063783416090031
8 sg:pub.10.1134/s1063783418020026
9 schema:datePublished 2019-03
10 schema:datePublishedReg 2019-03-01
11 schema:description The kinetics of near-edge photoluminescence (PL) in ZnO nanofilms prepared by the atomic layer deposition has been investigated. It is established that the kinetics of near-edge PL in 4-nm films is determined to a great extent by surface 2D-exciton (SX) and biexciton (SXX) complexes. The contribution from surface biexcitons is estimated based on a photostimulated change in the surface potential in ZnO films with different thicknesses. Ultrafast dynamics of surface biexcitons in thin films are revealed. It is shown that biexcitons localized near the surface have the shortest radiative lifetime (less than 100 ps) among all bound exciton complexes, which is explained by the large oscillator strength.
12 schema:genre article
13 schema:inLanguage en
14 schema:isAccessibleForFree false
15 schema:isPartOf Nb0e93c3af4f643bbb62de5bcd656f233
16 Nea12ee360de64b159e1b7afa0cba4361
17 sg:journal.1136591
18 schema:keywords ZnO films
19 ZnO nanofilms
20 ZnO thin films
21 atomic layer deposition
22 biexciton
23 biexciton complexes
24 changes
25 complexes
26 contribution
27 deposition
28 different thicknesses
29 dynamics
30 emission kinetics
31 exciton complexes
32 extent
33 films
34 greater extent
35 kinetics
36 large oscillator strength
37 layer deposition
38 lifetime
39 nanofilms
40 oscillator strengths
41 photoluminescence
42 photostimulated changes
43 potential
44 radiative lifetimes
45 short radiative lifetime
46 strength
47 surface
48 surface potential
49 thickness
50 thin films
51 ultrafast dynamics
52 schema:name Emission Kinetics of Surface (Bi)Excitons in ZnO Thin Films
53 schema:pagination 402-407
54 schema:productId N9098339c125b4e879f738f391062c439
55 Nbc28b47ddcd846f08b30dc940b849a4a
56 schema:sameAs https://app.dimensions.ai/details/publication/pub.1113627074
57 https://doi.org/10.1134/s1063783419030041
58 schema:sdDatePublished 2022-05-20T07:35
59 schema:sdLicense https://scigraph.springernature.com/explorer/license/
60 schema:sdPublisher N65f1e50c0df048d8aff84b75b225a000
61 schema:url https://doi.org/10.1134/s1063783419030041
62 sgo:license sg:explorer/license/
63 sgo:sdDataset articles
64 rdf:type schema:ScholarlyArticle
65 N036ebacc9eea4da6b22185002ec918e3 rdf:first sg:person.014034276053.56
66 rdf:rest N9a0dccafa5754cb096f202cc611fe736
67 N57fd6f520a1644be84ed1dba7bc0312d rdf:first sg:person.012314723253.70
68 rdf:rest N94af9399e05f4ad4b4d72297326f04aa
69 N65f1e50c0df048d8aff84b75b225a000 schema:name Springer Nature - SN SciGraph project
70 rdf:type schema:Organization
71 N9098339c125b4e879f738f391062c439 schema:name dimensions_id
72 schema:value pub.1113627074
73 rdf:type schema:PropertyValue
74 N94af9399e05f4ad4b4d72297326f04aa rdf:first sg:person.013444462541.44
75 rdf:rest N036ebacc9eea4da6b22185002ec918e3
76 N9a0dccafa5754cb096f202cc611fe736 rdf:first sg:person.0615207126.40
77 rdf:rest Nb083a545ab8f468797fb761694297070
78 Nb083a545ab8f468797fb761694297070 rdf:first sg:person.013312125473.62
79 rdf:rest Nb84c12bc19e24e3ba267c9c8ff525b7a
80 Nb0e93c3af4f643bbb62de5bcd656f233 schema:volumeNumber 61
81 rdf:type schema:PublicationVolume
82 Nb84c12bc19e24e3ba267c9c8ff525b7a rdf:first sg:person.014037377704.20
83 rdf:rest rdf:nil
84 Nbc28b47ddcd846f08b30dc940b849a4a schema:name doi
85 schema:value 10.1134/s1063783419030041
86 rdf:type schema:PropertyValue
87 Nea12ee360de64b159e1b7afa0cba4361 schema:issueNumber 3
88 rdf:type schema:PublicationIssue
89 anzsrc-for:02 schema:inDefinedTermSet anzsrc-for:
90 schema:name Physical Sciences
91 rdf:type schema:DefinedTerm
92 anzsrc-for:0203 schema:inDefinedTermSet anzsrc-for:
93 schema:name Classical Physics
94 rdf:type schema:DefinedTerm
95 anzsrc-for:0204 schema:inDefinedTermSet anzsrc-for:
96 schema:name Condensed Matter Physics
97 rdf:type schema:DefinedTerm
98 anzsrc-for:0206 schema:inDefinedTermSet anzsrc-for:
99 schema:name Quantum Physics
100 rdf:type schema:DefinedTerm
101 sg:grant.7595746 http://pending.schema.org/fundedItem sg:pub.10.1134/s1063783419030041
102 rdf:type schema:MonetaryGrant
103 sg:journal.1136591 schema:issn 0367-3294
104 1063-7834
105 schema:name Physics of the Solid State
106 schema:publisher Pleiades Publishing
107 rdf:type schema:Periodical
108 sg:person.012314723253.70 schema:affiliation grid-institutes:grid.15447.33
109 schema:familyName Akopyan
110 schema:givenName I. Kh.
111 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.012314723253.70
112 rdf:type schema:Person
113 sg:person.013312125473.62 schema:affiliation grid-institutes:grid.419569.6
114 schema:familyName Tomm
115 schema:givenName J. W.
116 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.013312125473.62
117 rdf:type schema:Person
118 sg:person.013444462541.44 schema:affiliation grid-institutes:grid.15447.33
119 schema:familyName Labzovskaya
120 schema:givenName M. E.
121 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.013444462541.44
122 rdf:type schema:Person
123 sg:person.014034276053.56 schema:affiliation grid-institutes:grid.15447.33
124 schema:familyName Novikov
125 schema:givenName B. V.
126 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.014034276053.56
127 rdf:type schema:Person
128 sg:person.014037377704.20 schema:affiliation grid-institutes:grid.9018.0
129 schema:familyName Schilling
130 schema:givenName J.
131 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.014037377704.20
132 rdf:type schema:Person
133 sg:person.0615207126.40 schema:affiliation grid-institutes:grid.9018.0
134 schema:familyName Talalaev
135 schema:givenName V. G.
136 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0615207126.40
137 rdf:type schema:Person
138 sg:pub.10.1007/978-3-642-10577-7 schema:sameAs https://app.dimensions.ai/details/publication/pub.1038674452
139 https://doi.org/10.1007/978-3-642-10577-7
140 rdf:type schema:CreativeWork
141 sg:pub.10.1134/s1063783416090031 schema:sameAs https://app.dimensions.ai/details/publication/pub.1019743702
142 https://doi.org/10.1134/s1063783416090031
143 rdf:type schema:CreativeWork
144 sg:pub.10.1134/s1063783418020026 schema:sameAs https://app.dimensions.ai/details/publication/pub.1101289295
145 https://doi.org/10.1134/s1063783418020026
146 rdf:type schema:CreativeWork
147 grid-institutes:grid.15447.33 schema:alternateName St. Petersburg State University, 199034, St. Petersburg, Russia
148 schema:name St. Petersburg State University, 199034, St. Petersburg, Russia
149 rdf:type schema:Organization
150 grid-institutes:grid.419569.6 schema:alternateName Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Berlin, Germany
151 schema:name Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Berlin, Germany
152 rdf:type schema:Organization
153 grid-institutes:grid.9018.0 schema:alternateName Martin-Luther University, Centre for Innovation Competence SiLi-nano, Halle, Germany
154 schema:name Martin-Luther University, Centre for Innovation Competence SiLi-nano, Halle, Germany
155 rdf:type schema:Organization
 




Preview window. Press ESC to close (or click here)


...