Behavior of Cobalt and Rare-Earth Subsystems in Frustrated Cobaltites DyBaCo4O7 + x View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2018-12

AUTHORS

Z. A. Kazei, V. V. Snegirev, M. S. Stolyarenko, K. S. Pigalskii, L. P. Kozeeva, M. Yu. Kameneva, A. N. Lavrov

ABSTRACT

Structural, elastic, and magnetic properties of cobaltites DyBaCo4O7 + x produced by various technologies and distinguished by oxygen excess x are experimentally studied. It was found that rhombic distortion of the crystal structure of annealed stoichiometric samples with x = 0 results in frustration removal and elastic property anomalies in the TN region, caused by cobalt subsystem ordering. At an insignificant oxygen nonstoichiometry, no structural distortions occur in quenched samples, and anomalies in elastic characteristics in the TN region smooth and disappear. The studies of DyBaCo4O7 + x magnetic properties show that the rare-earth (RE) subsystem remains paramagnetic and its contribution exceeds the contribution of the Co-subsystem with strong antiferromagnetic couplings by an order of magnitude. The magnetic susceptibility of the stoichiometric sample does not exhibit an appreciable anomaly at TN, since cobalt subsystem ordering is not accompanied by the formation of a noticeable effective field on RE ions. More... »

PAGES

2507-2516

References to SciGraph publications

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URI

http://scigraph.springernature.com/pub.10.1134/s1063783419010128

DOI

http://dx.doi.org/10.1134/s1063783419010128

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111953559


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