Optical, dynamic, and electro-optical properties of poly(N-acryloyl-11-aminoundecanoic acid) in solutions View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2011-08

AUTHORS

N. V. Tsvetkov, L. N. Andreeva, E. V. Lebedeva, I. A. Strelina, A. A. Lezov, A. N. Podseval’nikova, N. G. Mikusheva, V. O. Ivanova, I. A. Makarov, I. M. Zorin, A. Yu. Bilibin

ABSTRACT

The optical, electro-optical, and dynamic characteristics of poly(N-acryloyl-11-aminoundecanoic acid) in organic solvents and of the sodium salt of its monomer in water were studied via the methods of flow birefringence, equilibrium and nonequilibrium electric birefringence, and dynamic light scattering. It is shown that, in aqueous solutions, the monomer forms coarse particles of both symmetric and asymmetric shapes. The linear dimensions of these particles are estimated from the data of translational and rotational diffusion. Polymer macromolecules in organic solvents feature negative anisotropy of optical polarizability. Contributions of optical microform and macroform effects to the observed flow birefringence are analyzed in detail. The intrinsic optical anisotropy of the monomer unit of the polymer, which correlates well with the corresponding values for comb-shaped polymers of a similar structure, is estimated. It is shown that polymer molecules lack marked intrinsic permanent macromolecular dipoles and that electric birefringence in their solutions is associated with macroscopic induced dipole moments that appear during orientation of the dipole moments of polar groups in side chains of the polymer under application of an electric field. More... »

PAGES

666

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0965545x11080104

DOI

http://dx.doi.org/10.1134/s0965545x11080104

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1052793643


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