Zinc-Modified ZSM-5 Nanozeolites Synthesized by the Seed-Induced Method: Interrelation of Their Textural, Acidic, and Catalytic Properties in DME Conversion to ... View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2017-12

AUTHORS

Ke Zhang, S. A. Kurumov, Xiaofang Su, Yu. M. Snatenkova, Z. M. Bukina, N. V. Kolesnichenko, Wei Wu, S. N. Khadzhiev

ABSTRACT

The effect of the method of introduction of zinc cations and the zinc content in a nanocrystalline zeolite of the ZSM-5 type on the physicochemical and catalytic properties of the material in DME conversion to a mixture of liquid synthetic hydrocarbons has been studied. Zinc is introduced into the catalysts both during the zeolite synthesis and the ion exchange (ZnnAlmNZ5 and ZnNZ5, respectively). The use of nanocrystalline ZnnAlmNZ5 zeolites provides the formation of a mixture of liquid hydrocarbons with a high selectivity of no less than 90%; the liquid hydrocarbons contain more than 70% of isoparaffins and a small amount of aromatic compounds. An increase in the zinc loading of the ZnnAlmNZ5 zeolite from 0.9 to ~3% leads to an increase in the methanol content in the aqueous phase of the liquid product, an increase in the selectivity for liquid hydrocarbons, and a slight increase in the concentration of aromatic and unsaturated hydrocarbons in the mixture. In the presence of the ZnNZ5/Al2O3 catalyst with Zn introduced by ion exchange, the methanol content in the aqueous phase and the aromatics content in the liquid hydrocarbon mixture are significantly higher. The ZnnAlmNZ5 nanozeolites are characterized by a more developed external surface, a higher concentration of mesopores, and higher acidity. More... »

PAGES

1036-1042

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0965544117120179

DOI

http://dx.doi.org/10.1134/s0965544117120179

DIMENSIONS

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