Deactivation features of gallium-containing zeolites in the propane aromatization process View Full Text


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Article Info

DATE

2017-01

AUTHORS

L. N. Vosmerikova, V. I. Zaikovskii, A. N. Volynkina, A. V. Vosmerikov

ABSTRACT

Conversion of propane to aromatic hydrocarbons on Ga-containing zeolite catalysts prepared by various methods has been examined, and their comparative stability against deactivation has been analyzed. It has been shown that the Ga-containing zeolite catalysts exhibit high activity and stability in propane conversion to aromatic hydrocarbons. Specific features of the formation of carbon deposits on the surface of Ga-containing zeolites in the propane aromatization reaction have been revealed using the techniques of temperature-programmed desorption of ammonia, low-temperature adsorption of nitrogen, differential thermal analysis, high-resolution transmission electron microscopy, and characteristic X-ray spectroscopy radiation. It has been found that the coke deposited on the catalyst has an almost homogeneous structure and is characterized by relatively low degree of polycondensation. More... »

PAGES

85-92

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0965544116090231

DOI

http://dx.doi.org/10.1134/s0965544116090231

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1083763340


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