Synergistic effect of gold and copper in the catalytic conversion of ethanol to linear α-alcohols View Full Text


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Article Info

DATE

2016-08

AUTHORS

S. A. Nikolaev, A. V. Chistyakov, P. A. Zharova, M. V. Tsodikov, I. N. Krotova, D. I. Ezzgelenko

ABSTRACT

The reaction features of the direct conversion of ethanol to butanol-1 and hexanol-1 in the presence of mono- and bimetallic active components based on Au and Cu supported on γ-Al2O3 have been studied. It has been found that under conditions providing the supercritical state of ethanol, the reaction rate and selectivity in the presence of the Au–Cu/Al2O3 catalyst abruptly increases. In addition, a synergistic effect is observed: the yield of desired products over the Au–Cu catalyst is 6 or 14 times that over the Au or Cu monometallic counterpart, respectively. Differences in the catalytic behavior of the Au–Cu, Au-, and Cu-based systems have been discussed taking into account their structural features and the reaction mechanism. More... »

PAGES

730-737

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0965544116080120

DOI

http://dx.doi.org/10.1134/s0965544116080120

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1022447639


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