Hydrogenation of aromatic hydrocarbons over nickel–tungsten sulfide catalysts containing mesoporous aluminosilicates of different nature View Full Text


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Article Info

DATE

2016-07

AUTHORS

E. R. Naranov, A. S. Badeeva, A. A. Sadovnikov, S. V. Kardashev, A. L. Maksimov, S. V. Lysenko, V. A. Vinokurov, E. A. Karakhanov

ABSTRACT

The hydrogenation of naphthalene, toluene, and 2-methylnaphthalene used as model compounds; the hydrodearomatization of the methylnaphthalene fraction; and the hydrocracking of oil sludge over Ni–W sulfide catalysts supported on BEA/TUD, BEA/SBA-15, and ZSM-5/SBA-15 composites containing SBA-15 and TUD mesoporous silicates have been studied. Catalytic tests have been conducted in an autoclave at 300–400°C and an initial hydrogen pressure of 50–90 atm. It has been found that the highest activity is exhibited by the catalyst based on the ZSM-5/SBA-15 (1) composite prepared by the double-templating synthesis and characterized by a specific surface area of 400 m2/g and an acidity of 409 μmol/g. Thus, in the case of dearomatization of the methylnaphthalene fraction at 300°C and an H2 pressure of 50 atm, the content of diaromatic compounds has decreased from 99.0 to 53.4%, while the amount of sulfur compounds has decreased almost 15-fold. The hydrocracking of oil sludge over NiW/ZSM-5/SBA-15 (2) at 400°C and an H2 pressure of 90 atm has led to an increase in the content of light fractions to 52%. More... »

PAGES

599-606

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0965544116070124

DOI

http://dx.doi.org/10.1134/s0965544116070124

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1048401065


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