Theoretical aspects of methanol carbonylation on copper-containing zeolites View Full Text


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Article Info

DATE

2016-03

AUTHORS

A. A. Rybakov, I. A. Bryukhanov, A. V. Larin, G. M. Zhidomirov

ABSTRACT

The experimental data have been considered to match the theoretical mechanisms proposed previously to describe processes of oxidative carbonylation of methanol on copper-containing catalysts. The schemes examined cover methoxy intermediates, carbomethoxy intermediates, carbonates, and Cu(OCH3)2Cu binuclear clusters. The attack of the first methanol molecule on copper carbonate has been simulated in terms of the isolated cluster (8R) model with periodic boundary conditions (on CuMOR zeolite), and parameters of the individual steps involving description of the transition states have been evaluated. More... »

PAGES

259-266

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0965544116030129

DOI

http://dx.doi.org/10.1134/s0965544116030129

DIMENSIONS

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