Conversion of bio-oxygenates into hydrocarbons in the presence of a commercial Pt–Re/Al2O3 catalyst View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2016-11

AUTHORS

A. V. Chistyakov, P. A. Zharova, A. E. Gekhman, V. V. Kriventsov, M. V. Tsodikov

ABSTRACT

It was found that the preliminarily reduced commercial platinum–rhenium catalyst PR-71 exhibited high activity in the conversion of ethanol into C4–C12 olefins and in the cross-condensation reactions of ethanol with glycerol, acetone, n-propanol, and isopropanol. Acetone and glycerol exhibited the highest reactivity in the cross-condensation reactions; this manifested itself in an increase in the total yield of the target fraction of C4–C12 hydrocarbons and in a more than 10-fold increase in the yield of products containing the odd numbers of carbon atoms, as compared with the conversion of individual ethanol. The structural studies performed by extended X-ray absorption fine structure (EXAFS) spectroscopy and transmission electron microscopy showed that the high selectivity of PR-71 can be caused by the formation of bimetallic Pt–Re and Pt–Al clusters in the course of the prolonged preliminary reduction of the catalyst. More... »

PAGES

812-820

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0023158416060033

DOI

http://dx.doi.org/10.1134/s0023158416060033

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1038882816


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