Nonoxidative conversion of methane and n-pentane over a platinum/alumina catalyst View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2016-07

AUTHORS

D. V. Golinskii, N. V. Vinichenko, V. V. Pashkov, I. E. Udras, O. V. Krol’, V. P. Talzi, A. S. Belyi

ABSTRACT

Methane adsorption on the Pt–H/Al2O3 and Pt/Al2O3 catalysts begins at Т = 475°C and is accompanied by the appearance of hydrogen in the reaction medium. At a higher temperature is raised to 550°C, the amount of adsorbed hydrogen increases to 1.1 and 0.8 mol/(mol Pt), respectively. According to the calculated degree of methane dehydrogenation on platinum sites at Т = 550°C, the Н/C ratio is 1.3 (at/at) for the Pt–H/Al2O3 catalyst and 1.5 (at/at) for the Pt/Al2O3 catalyst. The introduction of n-pentane into the reaction medium increases the yield of aromatic hydrocarbons (benzene and toluene) by a factor of 8.8 over the arene yield observed in individual n-pentane conversion. A mass spectrometric analysis of the arenes obtained with the Pt/Al2O3 catalyst has demonstrated that 37.5% of the adsorbed methane is involved in the methane–n-pentane coaromatization yielding benzene and toluene. More... »

PAGES

504-510

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http://scigraph.springernature.com/pub.10.1134/s0023158416040042

DOI

http://dx.doi.org/10.1134/s0023158416040042

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