Polymetallic catalysts for the Fischer–Tropsch synthesis and hydrodesulfurization prepared using self-propagating high-temperature synthesis View Full Text


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Article Info

DATE

2015-09

AUTHORS

V. N. Borshch, E. V. Pugacheva, S. Ya. Zhuk, V. N. Sanin, D. E. Andreev, V. I. Yukhvid, O. L. Eliseev, R. V. Kazantsev, S. I. Kolesnikov, I. M. Kolesnikov, A. L. Lapidus

ABSTRACT

The synthesis, physicochemical characteristics, and operation of the previously proposed new multifunctional polymetallic catalysts in reduction processes are considered. The complex intermetallides of 3d metals and rare-earth elements, which are obtained by self-propagating high-temperature synthesis (SHS), are catalyst precursors. The catalyst structure includes a framework of lower intermetallic compounds covered with a strongly disordered highly amorphous metal oxide active phase. This phase forms two-level nanostructures (~10–100 nm) with a characteristic shape of flat hexahedrons on the surface. The catalysts possess high activity in the reactions of deep oxidation and reduction (the Fischer–Tropsch synthesis and the hydrodesulfurization of petroleum fractions); moreover, they do not require preliminary activation in the reduction processes. More... »

PAGES

681-688

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0023158415050031

DOI

http://dx.doi.org/10.1134/s0023158415050031

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1037390173


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