Ontology type: schema:ScholarlyArticle
2011-12
AUTHORSR. V. Gulyaev, L. S. Kibis, O. A. Stonkus, A. V. Zadesenets, P. E. Plyusnin, Yu. V. Shubin, S. V. Korenev, A. S. Ivanova, E. M. Slavinskaya, V. I. Zaikovskii, I. G. Danilova, A. I. Boronin, V. A. Sobyanin
ABSTRACTGold-palladium catalysts supported on cerium oxide were synthesized with the double complex salts. X-ray photoelectron spectroscopy (XPS) and other physicochemical methods (TEM, TPR) were used to demonstrate that synthesis of highly active palladium catalysts requires the oxidative treatment stimulating the formation of a catalytically active surface solid solution PdxCe1−xO2, which is responsible for the lowtemperature activity (LTA) in the reaction CO + O2. In the case of gold catalysts, active sites for the lowtemperature oxidation of CO are represented by gold nanoparticles and its cationic interface species. Simultaneous deposition of two metals increases the catalyst LTA due to interaction of both gold and palladium with the support surface to form a Pd1−xCexO2 solid solution and cationic interface species of palladium and gold on the boundary of Pd-Au alloy particles anchored on the solid solution surface. More... »
PAGES123-136
http://scigraph.springernature.com/pub.10.1134/s0022476611070171
DOIhttp://dx.doi.org/10.1134/s0022476611070171
DIMENSIONShttps://app.dimensions.ai/details/publication/pub.1007329357
JSON-LD is the canonical representation for SciGraph data.
TIP: You can open this SciGraph record using an external JSON-LD service: JSON-LD Playground Google SDTT
[
{
"@context": "https://springernature.github.io/scigraph/jsonld/sgcontext.json",
"about": [
{
"id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/03",
"inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/",
"name": "Chemical Sciences",
"type": "DefinedTerm"
},
{
"id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0306",
"inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/",
"name": "Physical Chemistry (incl. Structural)",
"type": "DefinedTerm"
}
],
"author": [
{
"affiliation": {
"alternateName": "G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.415877.8",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Gulyaev",
"givenName": "R. V.",
"id": "sg:person.01072673672.25",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01072673672.25"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.415877.8",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Kibis",
"givenName": "L. S.",
"id": "sg:person.010233564173.03",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010233564173.03"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.415877.8",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Stonkus",
"givenName": "O. A.",
"id": "sg:person.010735337041.08",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010735337041.08"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "A. V. Nikolaev Institute of Inorganic Chemistry, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.425759.8",
"name": [
"A. V. Nikolaev Institute of Inorganic Chemistry, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Zadesenets",
"givenName": "A. V.",
"id": "sg:person.012051546133.37",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.012051546133.37"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "Novosibirsk State University, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.4605.7",
"name": [
"A. V. Nikolaev Institute of Inorganic Chemistry, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"Novosibirsk State University, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Plyusnin",
"givenName": "P. E.",
"id": "sg:person.0643531001.56",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0643531001.56"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "Novosibirsk State University, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.4605.7",
"name": [
"A. V. Nikolaev Institute of Inorganic Chemistry, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"Novosibirsk State University, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Shubin",
"givenName": "Yu. V.",
"id": "sg:person.012641166115.54",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.012641166115.54"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "Novosibirsk State University, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.4605.7",
"name": [
"A. V. Nikolaev Institute of Inorganic Chemistry, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"Novosibirsk State University, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Korenev",
"givenName": "S. V.",
"id": "sg:person.0713211235.58",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0713211235.58"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.415877.8",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Ivanova",
"givenName": "A. S.",
"id": "sg:person.014116242012.51",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.014116242012.51"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.415877.8",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Slavinskaya",
"givenName": "E. M.",
"id": "sg:person.016045447241.09",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.016045447241.09"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.415877.8",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Zaikovskii",
"givenName": "V. I.",
"id": "sg:person.0770401015.84",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0770401015.84"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.415877.8",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Danilova",
"givenName": "I. G.",
"id": "sg:person.0741574275.56",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0741574275.56"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "Novosibirsk State University, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.4605.7",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"Novosibirsk State University, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Boronin",
"givenName": "A. I.",
"id": "sg:person.01272373255.22",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01272373255.22"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "Novosibirsk State University, Novosibirsk, Russia",
"id": "http://www.grid.ac/institutes/grid.4605.7",
"name": [
"G. K. Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, Novosibirsk, Russia",
"Novosibirsk State University, Novosibirsk, Russia"
],
"type": "Organization"
},
"familyName": "Sobyanin",
"givenName": "V. A.",
"id": "sg:person.011055206076.39",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.011055206076.39"
],
"type": "Person"
}
],
"citation": [
{
"id": "sg:pub.10.1023/a:1015352223861",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1000693729",
"https://doi.org/10.1023/a:1015352223861"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1134/s0023158410010246",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1019057580",
"https://doi.org/10.1134/s0023158410010246"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1023/a:1021428003587",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1006162246",
"https://doi.org/10.1023/a:1021428003587"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1007/s10562-008-9630-2",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1049283503",
"https://doi.org/10.1007/s10562-008-9630-2"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1007/s10562-006-0064-4",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1042568666",
"https://doi.org/10.1007/s10562-006-0064-4"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1007/bf01426965",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1032446082",
"https://doi.org/10.1007/bf01426965"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1007/s11244-007-9036-1",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1047854459",
"https://doi.org/10.1007/s11244-007-9036-1"
],
"type": "CreativeWork"
}
],
"datePublished": "2011-12",
"datePublishedReg": "2011-12-01",
"description": "Gold-palladium catalysts supported on cerium oxide were synthesized with the double complex salts. X-ray photoelectron spectroscopy (XPS) and other physicochemical methods (TEM, TPR) were used to demonstrate that synthesis of highly active palladium catalysts requires the oxidative treatment stimulating the formation of a catalytically active surface solid solution PdxCe1\u2212xO2, which is responsible for the lowtemperature activity (LTA) in the reaction CO + O2. In the case of gold catalysts, active sites for the lowtemperature oxidation of CO are represented by gold nanoparticles and its cationic interface species. Simultaneous deposition of two metals increases the catalyst LTA due to interaction of both gold and palladium with the support surface to form a Pd1\u2212xCexO2 solid solution and cationic interface species of palladium and gold on the boundary of Pd-Au alloy particles anchored on the solid solution surface.",
"genre": "article",
"id": "sg:pub.10.1134/s0022476611070171",
"inLanguage": "en",
"isAccessibleForFree": false,
"isPartOf": [
{
"id": "sg:journal.1135923",
"issn": [
"0022-4766",
"2542-0976"
],
"name": "Journal of Structural Chemistry",
"publisher": "Pleiades Publishing",
"type": "Periodical"
},
{
"issueNumber": "Suppl 1",
"type": "PublicationIssue"
},
{
"type": "PublicationVolume",
"volumeNumber": "52"
}
],
"keywords": [
"interface species",
"gold\u2013palladium catalysts",
"active palladium catalyst",
"double complex salts",
"Pd-Au alloy particles",
"solid solution surface",
"ray photoelectron spectroscopy",
"surface solid solution",
"low-temperature oxidation",
"gold catalysts",
"solid solution",
"gold nanoparticles",
"palladium catalyst",
"photoelectron spectroscopy",
"complex salts",
"physicochemical methods",
"oxidative treatment",
"active site",
"cerium oxide",
"reaction CO",
"catalyst",
"synergetic effect",
"solution surface",
"support surface",
"alloy particles",
"simultaneous deposition",
"palladium",
"CO",
"oxidation",
"gold",
"nanoparticles",
"spectroscopy",
"CeO2",
"surface",
"synthesis",
"salt",
"solution",
"oxide",
"O2",
"metals",
"deposition",
"particles",
"formation",
"species",
"interaction",
"sites",
"activity",
"method",
"effect",
"treatment",
"cases",
"boundaries"
],
"name": "Synergetic effect in PdAu/CeO2 catalysts for the low-temperature oxidation of CO",
"pagination": "123-136",
"productId": [
{
"name": "dimensions_id",
"type": "PropertyValue",
"value": [
"pub.1007329357"
]
},
{
"name": "doi",
"type": "PropertyValue",
"value": [
"10.1134/s0022476611070171"
]
}
],
"sameAs": [
"https://doi.org/10.1134/s0022476611070171",
"https://app.dimensions.ai/details/publication/pub.1007329357"
],
"sdDataset": "articles",
"sdDatePublished": "2022-05-20T07:26",
"sdLicense": "https://scigraph.springernature.com/explorer/license/",
"sdPublisher": {
"name": "Springer Nature - SN SciGraph project",
"type": "Organization"
},
"sdSource": "s3://com-springernature-scigraph/baseset/20220519/entities/gbq_results/article/article_526.jsonl",
"type": "ScholarlyArticle",
"url": "https://doi.org/10.1134/s0022476611070171"
}
]
Download the RDF metadata as: json-ld nt turtle xml License info
JSON-LD is a popular format for linked data which is fully compatible with JSON.
curl -H 'Accept: application/ld+json' 'https://scigraph.springernature.com/pub.10.1134/s0022476611070171'
N-Triples is a line-based linked data format ideal for batch operations.
curl -H 'Accept: application/n-triples' 'https://scigraph.springernature.com/pub.10.1134/s0022476611070171'
Turtle is a human-readable linked data format.
curl -H 'Accept: text/turtle' 'https://scigraph.springernature.com/pub.10.1134/s0022476611070171'
RDF/XML is a standard XML format for linked data.
curl -H 'Accept: application/rdf+xml' 'https://scigraph.springernature.com/pub.10.1134/s0022476611070171'
This table displays all metadata directly associated to this object as RDF triples.
230 TRIPLES
22 PREDICATES
85 URIs
70 LITERALS
6 BLANK NODES