Efficient step-mediated intercalation of silver atoms deposited on the Bi2Se3 surface View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2013-02-28

AUTHORS

M. M. Otrokov, S. D. Borisova, V. Chis, M. G. Vergniory, S. V. Eremeev, V. M. Kuznetsov, E. V. Chulkov

ABSTRACT

The intercalation of silver atoms into the van der Waals gap of the prototypical three-dimensional topological insulator Bi2Se3 is studied by means of ab initio total-energy calculations. Two possible intercalation mechanisms are examined: penetration from the terrace under the step and penetration via interstitials and/or vacancies of the surface quintuple layer block. It is shown that the former mechanism is strongly preferred over the latter one due to significant energy gain appearing at the step. According to performed estimations, the room temperature diffusion length of silver atoms reaches ten microns within a couple of minutes both on the surface and within the van der Waals gap, which essentially exceeds a typical distance between steps. These results shed light on the mechanism of intercalation of metal atoms deposited on the Bi2Se3 surface. More... »

PAGES

714-718

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0021364012230117

DOI

http://dx.doi.org/10.1134/s0021364012230117

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1005371755


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186 schema:name Institute of Strength Physics and Materials Science, Siberian Branch, Russian Academy of Sciences, 634021, Tomsk, Russia
187 Tomsk State University, 634050, Tomsk, Russia
188 rdf:type schema:Organization
189 grid-institutes:grid.77602.34 schema:alternateName Tomsk State University, 634050, Tomsk, Russia
190 schema:name Tomsk State University, 634050, Tomsk, Russia
191 rdf:type schema:Organization
 




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