Magnetic properties of Pr2–xFe1 + xSbO7 and Bi2–xLnxFeSbO7 (Ln = La, Pr) pyrochlore solid solutions View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2016-10

AUTHORS

A. V. Egorysheva, O. G. Ellert, O. M. Gaitko, A. A. Berseneva, Yu. V. Maksimov, T. D. Dudkina

ABSTRACT

The Bi–La–Fe–Sb–O, Pr–Fe–Sb–O, and Bi–Pr–Fe–Sb–O systems have been shown to contain pyrochlore solid solutions. We have determined the limits of the Pr2–xFe1 + xSbO7 and Bi2–xLnxFeSbO7 (Ln = La, Pr) solid solutions and shown that there is no compound corresponding to the “ideal” composition Pr2FeSbO7. Analysis of the magnetic properties of the synthesized compounds indicates that rare earth substitution for bismuth ions has no effect on the spin glass transition and that the spin glass state is only determined by the interaction between the Fe3+ spins on the octahedral site. The Pr3+ paramagnetic ion in Pr2–xFe1 + xSbO7 does not participate in the formation of the spin glass state but makes a paramagnetic contribution to the total magnetic susceptibility, which is especially significant at low temperatures. More... »

PAGES

1035-1044

Journal

TITLE

Inorganic Materials

ISSUE

10

VOLUME

52

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1134/s0020168516100071

DOI

http://dx.doi.org/10.1134/s0020168516100071

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1008102872


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