Polarization twist in perovskite ferrielectrics View Full Text


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Article Info

DATE

2016-10

AUTHORS

Yuuki Kitanaka, Kiyotaka Hirano, Motohiro Ogino, Yuji Noguchi, Masaru Miyayama, Chikako Moriyoshi, Yoshihiro Kuroiwa

ABSTRACT

Because the functions of polar materials are governed primarily by their polarization response to external stimuli, the majority of studies have focused on controlling polar lattice distortions. In some perovskite oxides, polar distortions coexist with nonpolar tilts and rotations of oxygen octahedra. The interplay between nonpolar and polar instabilities appears to play a crucial role, raising the question of how to design materials by exploiting their coupling. Here, we introduce the concept of 'polarization twist', which offers enhanced control over piezoelectric responses in polar materials. Our experimental and theoretical studies provide direct evidence that a ferrielectric perovskite exhibits a large piezoelectric response because of extended polar distortion, accompanied by nonpolar octahedral rotations, as if twisted polarization relaxes under electric fields. The concept underlying the polarization twist opens new possibilities for developing alternative materials in bulk and thin-film forms. More... »

PAGES

32216

References to SciGraph publications

Journal

TITLE

Scientific Reports

ISSUE

1

VOLUME

6

From Grant

  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/srep32216

    DOI

    http://dx.doi.org/10.1038/srep32216

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1028581209

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/27586824


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