Probing local and electronic structure in Warm Dense Matter: single pulse synchrotron x-ray absorption spectroscopy on shocked Fe View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-06-01

AUTHORS

Raffaella Torchio, Florent Occelli, Olivier Mathon, Arnaud Sollier, Emilien Lescoute, Laurent Videau, Tommaso Vinci, Alessandra Benuzzi-Mounaix, Jon Headspith, William Helsby, Simon Bland, Daniel Eakins, David Chapman, Sakura Pascarelli, Paul Loubeyre

ABSTRACT

Understanding Warm Dense Matter (WDM), the state of planetary interiors, is a new frontier in scientific research. There exists very little experimental data probing WDM states at the atomic level to test current models and those performed up to now are limited in quality. Here, we report a proof-of-principle experiment that makes microscopic investigations of materials under dynamic compression easily accessible to users and with data quality close to that achievable at ambient. Using a single 100 ps synchrotron x-ray pulse, we have measured, by K-edge absorption spectroscopy, ns-lived equilibrium states of WDM Fe. Structural and electronic changes in Fe are clearly observed for the first time at such extreme conditions. The amplitude of the EXAFS oscillations persists up to 500 GPa and 17000 K, suggesting an enduring local order. Moreover, a discrepancy exists with respect to theoretical calculations in the value of the energy shift of the absorption onset and so this comparison should help to refine the approximations used in models. More... »

PAGES

26402

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep26402

DOI

http://dx.doi.org/10.1038/srep26402

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1036914006

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/27246145


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