Competing coexisting phases in 2D water View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-05-17

AUTHORS

Jean-Marc Zanotti, Patrick Judeinstein, Simona Dalla-Bernardina, Gaëlle Creff, Jean-Blaise Brubach, Pascale Roy, Marco Bonetti, Jacques Ollivier, Dimitrios Sakellariou, Marie-Claire Bellissent-Funel

ABSTRACT

The properties of bulk water come from a delicate balance of interactions on length scales encompassing several orders of magnitudes: i) the Hydrogen Bond (HBond) at the molecular scale and ii) the extension of this HBond network up to the macroscopic level. Here, we address the physics of water when the three dimensional extension of the HBond network is frustrated, so that the water molecules are forced to organize in only two dimensions. We account for the large scale fluctuating HBond network by an analytical mean-field percolation model. This approach provides a coherent interpretation of the different events experimentally (calorimetry, neutron, NMR, near and far infra-red spectroscopies) detected in interfacial water at 160, 220 and 250 K. Starting from an amorphous state of water at low temperature, these transitions are respectively interpreted as the onset of creation of transient low density patches of 4-HBonded molecules at 160 K, the percolation of these domains at 220 K and finally the total invasion of the surface by them at 250 K. The source of this surprising behaviour in 2D is the frustration of the natural bulk tetrahedral local geometry and the underlying very significant increase in entropy of the interfacial water molecules. More... »

PAGES

25938

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep25938

DOI

http://dx.doi.org/10.1038/srep25938

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1005166985

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/27185018


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