Supramolecular One-Dimensional n/p-Nanofibers View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2015-11

AUTHORS

Alberto Insuasty, Carmen Atienza, Juan Luis López, Juan Marco-Martínez, Santiago Casado, Avishek Saha, Dirk M Guldi, Nazario Martín

ABSTRACT

Currently, there is a broad interest in the control over creating ordered electroactive nanostructures, in which electron donors and acceptors are organized at similar length scales. In this article, a simple and efficient procedure is reported en-route towards the construction of 1D arrays of crystalline pristine C60 and phenyl-C61-butyric acid methyl ester (PCBM) coated onto supramolecular fibers based on exTTF-pentapeptides. The resulting n/p-nanohybrids have been fully characterized by a variety of spectroscopic (FTIR, UV-Vis, circular dichroism, Raman and transient absorption), microscopic (AFM, TEM, and SEM), and powder diffraction (X-ray) techniques. Our experimental findings document the tendency of electroactive exTTF-fibers to induce the crystallization of C60 and PCBM, on one hand, and to afford 1D n/p-nanohybrids, on the other hand. Furthermore, photogenerated radical ion pairs, formed upon visible light irradiation of the n/p-nanohybrids, feature lifetimes on the range of 0.9-1.2 ns. More... »

PAGES

14154

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep14154

DOI

http://dx.doi.org/10.1038/srep14154

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1041910393

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26369586


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