Hierarchical multicolor nano-pixel matrices formed by coordinating luminescent metal ions to a conjugated poly(4′-octyl-2′,6′-bispyrazoyl pyridine) film via contact printing View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2015-07

AUTHORS

Supratim Basak, Ahamad Mohiddon, Martin Baumgarten, Klaus Müllen, Rajadurai Chandrasekar

ABSTRACT

We introduce a cost-effective, yet feasible reactive printing approach namely, "coordination chemistry at the conjugated ligand polymer surface". By using a contact printing technique we selectively fabricated high resolution nano-pixel configurations consisting of red, blue and green (R,G,B) colors arranged in a hierarchical three-dimensional fashion. For this, we have synthesized a novel blue emitting conjugated ligand polymer, [poly(4'-octyl-2',6'-bispyrazoyl pyridine)] ( ~ 7-8 KDa) having a tridentate ligand in its repeating unit which forms a thin film prone of binding metal ions. On top of this ligand polymer film, a layer of high-resolution cross-stripes (width ca. 800 nm) was printed comprised of Eu and Tb ions over a large area ~ 100 × 100 μm(2). The final woodpile-like assembly produced a new pixel group consisting of B; BG; BR; and BGR (White) colors. The area of the white emitting square is ca. 0.64 μm(2). The patterned layers that make up the pixels are very thin and thus this new technique might find applications in flexible light emitting devices. More... »

PAGES

8406

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep08406

DOI

http://dx.doi.org/10.1038/srep08406

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1042006709

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25673007


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