Ontology type: schema:ScholarlyArticle Open Access: True
2015-07
AUTHORSSofia Masi, Silvia Colella, Andrea Listorti, Vittoria Roiati, Andrea Liscio, Vincenzo Palermo, Aurora Rizzo, Giuseppe Gigli
ABSTRACTHere we conceive an innovative nanocomposite to endow hybrid perovskites with the easy processability of polymers, providing a tool to control film quality and material crystallinity. We verify that the employed semiconducting polymer, poly[2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene] (MEH-PPV), controls the self-assembly of CH₃NH₃PbI₃ (MAPbI₃) crystalline domains and favors the deposition of a very smooth and homogenous layer in one straightforward step. This idea offers a new paradigm for the implementation of polymer/perovskite nanocomposites towards versatile optoelectronic devices combined with the feasibility of mass production. As a proof-of-concept we propose the application of such nanocomposite in polymer solar cell architecture, demonstrating a power conversion efficiency up to 3%, to date the highest reported for MEH-PPV. On-purpose designed polymers are expected to suit the nanocomposite properties for the integration in diverse optoelectronic devices via facile processing condition. More... »
PAGES7725
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DOIhttp://dx.doi.org/10.1038/srep07725
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