Spin-orbit coupling induced semi-metallic state in the 1/3 hole-doped hyper-kagome Na3Ir3O8 View Full Text


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Article Info

DATE

2015-05

AUTHORS

Tomohiro Takayama, Alexander Yaresko, Akiyo Matsumoto, Jürgen Nuss, Kenji Ishii, Masahiro Yoshida, Junichiro Mizuki, Hidenori Takagi

ABSTRACT

The complex iridium oxide Na3Ir3O8 with a B-site ordered spinel structure was synthesized in single crystalline form, where the chiral hyper-kagome lattice of Ir ions, as observed in the spin-liquid candidate Na4Ir3O8, was identified. The average valence of Ir is 4.33+ and, therefore, Na3Ir3O8 can be viewed as a doped analogue of the hyper-kagome spin liquid with Ir(4+). The transport measurements, combined with the electronic structure calculations, indicate that the ground state of Na3Ir3O8 is a low carrier density semi-metal. We argue that the semi-metallic state is produced by a competition of the molecular orbital splitting of t2g orbitals on Ir3 triangles with strong spin-orbit coupling inherent to heavy Ir ions. More... »

PAGES

6818

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep06818

DOI

http://dx.doi.org/10.1038/srep06818

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https://app.dimensions.ai/details/publication/pub.1010691542

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25351992


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