Nanostructured organosilicon luminophores and their application in highly efficient plastic scintillators View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2014-10-08

AUTHORS

Sergei A. Ponomarenko, Nikolay M. Surin, Oleg V. Borshchev, Yuriy N. Luponosov, Dmitry Y. Akimov, Ivan S. Alexandrov, Alexander A. Burenkov, Alexey G. Kovalenko, Viktor N. Stekhanov, Elena A. Kleymyuk, Oleg T. Gritsenko, Georgiy V. Cherkaev, Alexander S. Kechek'yan, Olga A. Serenko, Aziz M. Muzafarov

ABSTRACT

Organic luminophores are widely used in various optoelectronic devices, which serve for photonics, nuclear and particle physics, quantum electronics, medical diagnostics and many other fields of science and technology. Improving their spectral-luminescent characteristics for particular technical requirements of the devices is a challenging task. Here we show a new concept to universal solution of this problem by creation of nanostructured organosilicon luminophores (NOLs), which are a particular type of dendritic molecular antennas. They combine the best properties of organic luminophores and inorganic quantum dots: high absorption cross-section, excellent photoluminescence quantum yield, fast luminescence decay time and good processability. A NOL consists of two types of covalently bonded via silicon atoms organic luminophores with efficient Förster energy transfer between them. Using NOLs in plastic scintillators, widely utilized for radiation detection and in elementary particles discoveries, led to a breakthrough in their efficiency, which combines both high light output and fast decay time. Moreover, for the first time plastic scintillators, which emit light in the desired wavelength region ranging from 370 to 700 nm, have been created. We anticipate further applications of NOLs as working elements of pulsed dye lasers in photonics, optoelectronics and as fluorescent labels in biology and medical diagnostics. More... »

PAGES

6549

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep06549

DOI

http://dx.doi.org/10.1038/srep06549

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1002594475

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25293808


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19 schema:description Organic luminophores are widely used in various optoelectronic devices, which serve for photonics, nuclear and particle physics, quantum electronics, medical diagnostics and many other fields of science and technology. Improving their spectral-luminescent characteristics for particular technical requirements of the devices is a challenging task. Here we show a new concept to universal solution of this problem by creation of nanostructured organosilicon luminophores (NOLs), which are a particular type of dendritic molecular antennas. They combine the best properties of organic luminophores and inorganic quantum dots: high absorption cross-section, excellent photoluminescence quantum yield, fast luminescence decay time and good processability. A NOL consists of two types of covalently bonded via silicon atoms organic luminophores with efficient Förster energy transfer between them. Using NOLs in plastic scintillators, widely utilized for radiation detection and in elementary particles discoveries, led to a breakthrough in their efficiency, which combines both high light output and fast decay time. Moreover, for the first time plastic scintillators, which emit light in the desired wavelength region ranging from 370 to 700 nm, have been created. We anticipate further applications of NOLs as working elements of pulsed dye lasers in photonics, optoelectronics and as fluorescent labels in biology and medical diagnostics.
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25 schema:keywords Förster energy transfer
26 absorption
27 antenna
28 applications
29 biology
30 breakthrough
31 challenging task
32 characteristics
33 concept
34 creation
35 decay time
36 detection
37 devices
38 diagnostics
39 discovery
40 dots
41 dye laser
42 efficiency
43 efficient Förster energy transfer
44 electronics
45 elements
46 energy transfer
47 excellent photoluminescence quantum yield
48 fast decay time
49 fast luminescence decay time
50 field
51 fields of science
52 fluorescent labels
53 further application
54 good processability
55 good properties
56 high absorption
57 high light output
58 inorganic quantum dots
59 labels
60 laser
61 light
62 light output
63 luminescence decay time
64 luminophores
65 medical diagnostics
66 molecular antenna
67 nanostructured organosilicon luminophores
68 new concept
69 optoelectronic devices
70 optoelectronics
71 organic luminophores
72 organosilicon
73 output
74 particle physics
75 particular type
76 photoluminescence quantum yield
77 photonics
78 physics
79 plastic scintillator
80 problem
81 processability
82 properties
83 quantum dots
84 quantum electronics
85 quantum yield
86 radiation detection
87 region
88 requirements
89 science
90 scintillator
91 silicon
92 solution
93 spectral-luminescent characteristics
94 task
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96 technology
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