Towards ultrahigh volumetric capacitance: graphene derived highly dense but porous carbons for supercapacitors View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-12

AUTHORS

Ying Tao, Xiaoying Xie, Wei Lv, Dai-Ming Tang, Debin Kong, Zhenghong Huang, Hirotomo Nishihara, Takafumi Ishii, Baohua Li, Dmitri Golberg, Feiyu Kang, Takashi Kyotani, Quan-Hong Yang

ABSTRACT

A small volumetric capacitance resulting from a low packing density is one of the major limitations for novel nanocarbons finding real applications in commercial electrochemical energy storage devices. Here we report a carbon with a density of 1.58 g cm(-3), 70% of the density of graphite, constructed of compactly interlinked graphene nanosheets, which is produced by an evaporation-induced drying of a graphene hydrogel. Such a carbon balances two seemingly incompatible characteristics: a porous microstructure and a high density, and therefore has a volumetric capacitance for electrochemical capacitors (ECs) up to 376 F cm(-3), which is the highest value so far reported for carbon materials in an aqueous electrolyte. More promising, the carbon is conductive and moldable, and thus could be used directly as a well-shaped electrode sheet for the assembly of a supercapacitor device free of any additives, resulting in device-level high energy density ECs. More... »

PAGES

2975

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep02975

DOI

http://dx.doi.org/10.1038/srep02975

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1027492146

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/24131954


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