Biopolymer-Activated Graphitic Carbon Nitride towards a Sustainable Photocathode Material View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-12

AUTHORS

Yuanjian Zhang, Zoë Schnepp, Junyu Cao, Shuxin Ouyang, Ying Li, Jinhua Ye, Songqin Liu

ABSTRACT

Photoelectrochemical (PEC) conversion of solar light into chemical fuels is one of the most promising solutions to the challenge of sustainable energy. Graphitic carbon (IV) nitride polymer (g-CN) is an interesting sustainable photocathode material due to low-cost, visible-light sensitivity, and chemical stability up to 500 °C in air. However, grain boundary effects and limited active sites greatly hamper g-CN activity. Here, we demonstrate biopolymer-activation of g-CN through simultaneous soft-templating of a sponge-like structure and incorporation of active carbon-dopant sites. This facile approach results in an almost 300% increase in the cathodic PEC activity of g-CN under simulated solar-irradiation. More... »

PAGES

2163

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep02163

DOI

http://dx.doi.org/10.1038/srep02163

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1034242794

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/23831846


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