Heteroepitaxial Growth of Single-Walled Carbon Nanotubes from Boron Nitride View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2012-12

AUTHORS

Dai-Ming Tang, Li-Li Zhang, Chang Liu, Li-Chang Yin, Peng-Xiang Hou, Hua Jiang, Zhen Zhu, Feng Li, Bilu Liu, Esko I. Kauppinen, Hui-Ming Cheng

ABSTRACT

The growth of single-walled carbon nanotubes (SWCNTs) with predefined structure is of great importance for both fundamental research and their practical applications. Traditionally, SWCNTs are grown from a metal catalyst with a vapor-liquid-solid mechanism, where the catalyst is in liquid state with fluctuating structures, and it is intrinsically unfavorable for the structure control of SWCNTs. Here we report the heteroepitaxial growth of SWCNTs from a platelet boron nitride nanofiber (BNNF), which is composed of stacked (002) planes and is stable at high temperatures. SWCNTs are found to grow epitaxially from the open (002) edges of the BNNFs, and the diameters of the SWCNTs are multiples of the BN (002) interplanar distance. In situ transmission electron microscopy observations coupled with first principles calculations reveal that the growth of SWCNTs from the BNNFs follows a vapor-solid-solid mechanism. Our work opens opportunities for the control over the structure of SWCNTs by hetero-crystallographic epitaxy. More... »

PAGES

971

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/srep00971

DOI

http://dx.doi.org/10.1038/srep00971

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1046940379

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/23240076


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