Paramagnetic gold in a highly disordered Au-Ni-O alloy View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-09-11

AUTHORS

A. Stamatelatos, P. Poulopoulos, A. Goschew, P. Fumagalli, E. Sarigiannidou, L. Rapenne, C. Opagiste, S. Grammatikopoulos, F. Wilhelm, A. Rogalev

ABSTRACT

Magnetic materials are usually classified into a distinct category such as diamagnets, paramagnets or ferromagnets. The enormous progress in materials science allows one nowadays, however, to change the magnetic nature of an element in a material. Gold, in bulk form, is traditionally a diamagnet. But in a ferromagnetic environment, it can adopt an induced ferromagnetic moment. Moreover, the growth of gold under certain conditions may lead to a spontaneous ferromagnetic or paramagnetic response. Here, we report on paramagnetic gold in a highly disordered Au-Ni-O alloy and focus on the unusual magnetic response. Such materials are mainly considered for plasmonic applications. Thin films containing Au, Ni and NiO are fabricated by co-deposition of Ni and Au in a medium vacuum of 2 × 10-2 mbar. As a result, Au is in a fully disordered state forming in some cases isolated nanocrystallites of up to 4 nm in diameter as revealed by high resolution transmission electron microscopy. The disorder and the environment, which is rich in oxygen, lead to remarkable magnetic properties of Au: an induced ferromagnetic and a paramagnetic state. This can be proven by measuring the x-ray magnetic circular dichroism. Our experiments show a way to establish and monitor Au paramagnetism in alloys. More... »

PAGES

13137

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-019-49457-7

DOI

http://dx.doi.org/10.1038/s41598-019-49457-7

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1120961815

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/31511624


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