Significant THz absorption in CH3NH2 molecular defect-incorporated organic-inorganic hybrid perovskite thin film. View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Inhee Maeng, Young Mi Lee, Jinwoo Park, Sonia R Raga, Chul Kang, Chul-Sik Kee, Byung Deok Yu, Suklyun Hong, Luis K Ono, Yabing Qi, Min-Cherl Jung, Masakazu Nakamura

ABSTRACT

The valid strong THz absorption at 1.58 THz was probed in the organic-inorganic hybrid perovskite thin film, CH3NH3PbI3, fabricated by sequential vacuum evaporation method. In usual solution-based methods such as 2-step solution and antisolvent, we observed the relatively weak two main absorption peaks at 0.95 and 1.87 THz. The measured absorption spectrum is analyzed by density-functional theory calculations. The modes at 0.95 and 1.87 THz are assigned to the Pb-I vibrations of the inorganic components in the tetragonal phase. By contrast, the origin of the 1.58 THz absorption is due to the structural deformation of Pb-I bonding at the grain boundary incorporated with a CH3NH2 molecular defect. More... »

PAGES

5811

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-019-42359-8

DOI

http://dx.doi.org/10.1038/s41598-019-42359-8

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1113327814

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30967593


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40 schema:description The valid strong THz absorption at 1.58 THz was probed in the organic-inorganic hybrid perovskite thin film, CH<sub>3</sub>NH<sub>3</sub>PbI<sub>3</sub>, fabricated by sequential vacuum evaporation method. In usual solution-based methods such as 2-step solution and antisolvent, we observed the relatively weak two main absorption peaks at 0.95 and 1.87 THz. The measured absorption spectrum is analyzed by density-functional theory calculations. The modes at 0.95 and 1.87 THz are assigned to the Pb-I vibrations of the inorganic components in the tetragonal phase. By contrast, the origin of the 1.58 THz absorption is due to the structural deformation of Pb-I bonding at the grain boundary incorporated with a CH<sub>3</sub>NH<sub>2</sub> molecular defect.
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