Magnetic and electronic properties of magnetite across the high pressure anomaly View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

D. P. Kozlenko, L. S. Dubrovinsky, S. E. Kichanov, E. V. Lukin, V. Cerantola, A. I. Chumakov, B. N. Savenko

ABSTRACT

The magnetite Fe3O4, being anciently known magnetic material to human kind and remaining in leading positions for development of advanced technologies presently, demonstrates a number of puzzling physical phenomena, being at focus of extensive research for more than century. Recently the pressure-induced anomalous behavior of physical properties of magnetite in vicinity of the structural phase transition, occurring at P ~ 25-30 GPa, has attracted particular attention, and its nature remains unclear. Here we study the magnetic and electronic properties of magnetite across high pressure anomaly and in the pressure-induced phase by means of 57Fe synchrotron Moessbauer spectroscopy and neutron diffraction. The hyperfine interaction parameters behavior was systematically analysed over pressure 0-40 GPa and temperature 10-290 K ranges. In the high pressure phase the ferrimagnetic order formation below TNP ~ 420 K was observed and spin arrangement symmetry was deduced. The structural, magnetic and electronic phase diagram of magnetite in the discussed pressure range is established. More... »

PAGES

4464

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-019-41184-3

DOI

http://dx.doi.org/10.1038/s41598-019-41184-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1112760760

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30872759


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43 schema:description The magnetite Fe<sub>3</sub>O<sub>4</sub>, being anciently known magnetic material to human kind and remaining in leading positions for development of advanced technologies presently, demonstrates a number of puzzling physical phenomena, being at focus of extensive research for more than century. Recently the pressure-induced anomalous behavior of physical properties of magnetite in vicinity of the structural phase transition, occurring at P ~ 25-30 GPa, has attracted particular attention, and its nature remains unclear. Here we study the magnetic and electronic properties of magnetite across high pressure anomaly and in the pressure-induced phase by means of <sup>57</sup>Fe synchrotron Moessbauer spectroscopy and neutron diffraction. The hyperfine interaction parameters behavior was systematically analysed over pressure 0-40 GPa and temperature 10-290 K ranges. In the high pressure phase the ferrimagnetic order formation below T<sub>NP</sub> ~ 420 K was observed and spin arrangement symmetry was deduced. The structural, magnetic and electronic phase diagram of magnetite in the discussed pressure range is established.
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