Degradation pathways in standard and inverted DBP-C70 based organic solar cells View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Golnaz Sherafatipour, Johannes Benduhn, Bhushan R. Patil, Mehrad Ahmadpour, Donato Spoltore, Horst-Günter Rubahn, Koen Vandewal, Morten Madsen

ABSTRACT

Achieving long-term stability in organic solar cells is a remaining bottleneck for the commercialization of this otherwise highly appealing technology. In this work, we study the performance and stability differences in standard and inverted DBP/C70 based organic solar cells. Differences in the charge-transfer state properties of inverted and standard configuration DBP/C70 solar cells are revealed by sensitive external quantum efficiency measurements, leading to differences in the open-circuit voltages of the devices. The degradation of standard and inverted solar cell configurations at ISOS aging test conditions (ISOS-D-3 and ISOS-T-3) was investigated and compared. The results indicate that the performance drop in the small molecule bilayer solar cells is less related to changes at the D-A interface, suggesting also a pronounced morphological stability, and instead, in the case of inverted cells, dominated by degradation at the electron transport layer (ETL) bathocuproine (BCP). Photoluminescence measurements, electron-only-device characteristics, and stability measurements show improved exciton blocking, electron transport properties and a higher stability for BCP/Ag ETL stacks, giving rise to inverted devices with enhanced performance and device stability. More... »

PAGES

4024

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-019-40541-6

DOI

http://dx.doi.org/10.1038/s41598-019-40541-6

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1112675903

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30858539


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