Multi-photon ionisation spectroscopy for rotational state preparation of N2+ View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-12

AUTHORS

Amy Gardner, Timothy Softley, Matthias Keller

ABSTRACT

In this paper we investigate the 2 + 1' resonance enhanced multi-photon ionisation (REMPI) of molecular nitrogen via the a1Πg(v = 6) intermediate state and analyse its feasibility to generate molecular nitrogen ions in a well defined ro-vibrational state. This is an important tool for high precision experiments based on trapped molecular ions, and is crucial for studying the time variation of the fundamental constant mp/me using [Formula: see text]. The transition is not reported in the literature and detailed spectral analysis has been conducted to extract the molecular constants of the intermediate state. By carefully choosing the intermediate ro-vibrational state, the ionisation laser wavelength and controlling the excitation laser pulse energy, unwanted formation of rotationally excited molecular ions can be suppressed and ro-vibrational ground state ions can be generated with high purity. More... »

PAGES

506

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-018-36783-5

DOI

http://dx.doi.org/10.1038/s41598-018-36783-5

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111635765

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30679634


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41 schema:description In this paper we investigate the 2 + 1' resonance enhanced multi-photon ionisation (REMPI) of molecular nitrogen via the a<sup>1</sup>Π<sub>g</sub>(v = 6) intermediate state and analyse its feasibility to generate molecular nitrogen ions in a well defined ro-vibrational state. This is an important tool for high precision experiments based on trapped molecular ions, and is crucial for studying the time variation of the fundamental constant m<sub>p</sub>/m<sub>e</sub> using [Formula: see text]. The transition is not reported in the literature and detailed spectral analysis has been conducted to extract the molecular constants of the intermediate state. By carefully choosing the intermediate ro-vibrational state, the ionisation laser wavelength and controlling the excitation laser pulse energy, unwanted formation of rotationally excited molecular ions can be suppressed and ro-vibrational ground state ions can be generated with high purity.
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