Femtosecond phase-transition in hard x-ray excited bismuth View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-01-24

AUTHORS

M. Makita, I. Vartiainen, I. Mohacsi, C. Caleman, A. Diaz, H. O. Jönsson, P. Juranić, N. Medvedev, A. Meents, A. Mozzanica, N. L. Opara, C. Padeste, V. Panneels, V. Saxena, M. Sikorski, S. Song, L. Vera, P. R. Willmott, P. Beaud, C. J. Milne, B. Ziaja-Motyka, C. David

ABSTRACT

The evolution of bismuth crystal structure upon excitation of its A1g phonon has been intensely studied with short pulse optical lasers. Here we present the first-time observation of a hard x-ray induced ultrafast phase transition in a bismuth single crystal at high intensities (~1014 W/cm2). The lattice evolution was followed using a recently demonstrated x-ray single-shot probing setup. The time evolution of the (111) Bragg peak intensity showed strong dependence on the excitation fluence. After exposure to a sufficiently intense x-ray pulse, the peak intensity dropped to zero within 300 fs, i.e. faster than one oscillation period of the A1g mode at room temperature. Our analysis indicates a nonthermal origin of a lattice disordering process, and excludes interpretations based on electron-ion equilibration process, or on thermodynamic heating process leading to plasma formation. More... »

PAGES

602

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-018-36216-3

DOI

http://dx.doi.org/10.1038/s41598-018-36216-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111646331

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30679456


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14 schema:description The evolution of bismuth crystal structure upon excitation of its A<sub>1g</sub> phonon has been intensely studied with short pulse optical lasers. Here we present the first-time observation of a hard x-ray induced ultrafast phase transition in a bismuth single crystal at high intensities (~10<sup>14</sup> W/cm<sup>2</sup>). The lattice evolution was followed using a recently demonstrated x-ray single-shot probing setup. The time evolution of the (111) Bragg peak intensity showed strong dependence on the excitation fluence. After exposure to a sufficiently intense x-ray pulse, the peak intensity dropped to zero within 300 fs, i.e. faster than one oscillation period of the A<sub>1g</sub> mode at room temperature. Our analysis indicates a nonthermal origin of a lattice disordering process, and excludes interpretations based on electron-ion equilibration process, or on thermodynamic heating process leading to plasma formation.
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