Revealing of Core Shell Effect on Frequency-Dependent Properties of Bi-based Relaxor/Ferroelectric Ceramic Composites View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Mohsin Saleem, Lim Dong Hwan, In-sung Kim, Min-Soo Kim, Adnan Maqbool, Umair Nisar, Syed Atif Pervez, Umer Farooq, Muhammad Umer Farooq, Hafiz Muhammad Waseem Khalil, Soon-Jong Jeong

ABSTRACT

In this study, electromechanical characteristics of (1-x) Bi0.5Na0.5TiO3-xSrTiO3 (ST26, x = 0.26)/(1-y) Bi0.5Na0.5TiO3-ySrTiO3 (ST10, y = 0.1) (matrix/seed) composites were studied. The ST26 (high relaxor phase) and ST10 (a relaxor ferroelectric (RF), high ferroelectric phase) composite with large (r-ST26-ST10) and small (t-ST26-ST10) grains exhibited frequency-related dielectric properties and large strain response at a low triggering electric field (an incipient piezoelectricity). It is ascribed to a matrix-seed effect originating from the inhomogeneous composition due to the presence of two phases. The r-ST26-ST10 composite sintered at 4 h, prominent material, showed a high normalized dynamic strain (d33*) of ~700 pm/V (large grains) with stable frequency dependence properties at a low field of 40 kV/cm. The properties of the r-ST26-ST10 composite exhibit less decay with frequency-related polarization and strain compared to those of t-ST26-ST10 composite. The increase in soaking time promotes the diffusion and homogenization of the microstructure in composites, leading to changes in the core-shell structure in the solid solution. The polarization and strain of the ST26-ST10 composites with the frequency are linked to the stability of the internal random fields created by non-ergodic relaxor phase of seed and the amount of phase change in the ergodic relaxor matrix. More... »

PAGES

14146

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-018-32133-7

DOI

http://dx.doi.org/10.1038/s41598-018-32133-7

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1106987094

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30237430


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