Kinked silicon nanowires-enabled interweaving electrode configuration for lithium-ion batteries View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Georgiana Sandu, Michael Coulombier, Vishank Kumar, Hailu G. Kassa, Ionel Avram, Ran Ye, Antoine Stopin, Davide Bonifazi, Jean-François Gohy, Philippe Leclère, Xavier Gonze, Thomas Pardoen, Alexandru Vlad, Sorin Melinte

ABSTRACT

A tri-dimensional interweaving kinked silicon nanowires (k-SiNWs) assembly, with a Ni current collector co-integrated, is evaluated as electrode configuration for lithium ion batteries. The large-scale fabrication of k-SiNWs is based on a procedure for continuous metal assisted chemical etching of Si, supported by a chemical peeling step that enables the reuse of the Si substrate. The kinks are triggered by a simple, repetitive etch-quench sequence in a HF and H2O2-based etchant. We find that the inter-locking frameworks of k-SiNWs and multi-walled carbon nanotubes exhibit beneficial mechanical properties with a foam-like behavior amplified by the kinks and a suitable porosity for a minimal electrode deformation upon Li insertion. In addition, ionic liquid electrolyte systems associated with the integrated Ni current collector repress the detrimental effects related to the Si-Li alloying reaction, enabling high cycling stability with 80% capacity retention (1695 mAh/gSi) after 100 cycles. Areal capacities of 2.42 mAh/cm2 (1276 mAh/gelectrode) can be achieved at the maximum evaluated thickness (corresponding to 1.3 mgSi/cm2). This work emphasizes the versatility of the metal assisted chemical etching for the synthesis of advanced Si nanostructures for high performance lithium ion battery electrodes. More... »

PAGES

9794

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-018-28108-3

DOI

http://dx.doi.org/10.1038/s41598-018-28108-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1105071673

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29955101


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