Thermooptical evidence of carrier-stabilized ferroelectricity in ultrathin electrodeless films View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

O. Pacherova, D. Chvostova, T. Kocourek, M. Jelinek, A. Dejneka, E. Eliseev, A. Morozovska, M. Tyunina

ABSTRACT

Ferroelectric films may lose polarization as their thicknesses decrease to a few nanometers because of the depolarizing field that opposes the polarization therein. The depolarizing field is minimized when electrons or ions in the electrodes or the surface/interface layers screen the polarization charge or when peculiar domain configuration is formed. Here, we demonstrate ferroelectric phase transitions using thermooptical studies in ∼5-nm-thick epitaxial Pb0.5Sr0.5TiO3 films grown on different insulating substrates. By comparing theoretical modeling and experimental observations, we show that ferroelectricity is stabilized through redistribution of charge carriers (electrons or holes) inside ultrathin films. The related high-density of screening carriers is confined within a few-nanometers-thick layer in the vicinity of the insulator, thus resembling a two-dimensional carrier gas. More... »

PAGES

8497

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-018-26933-0

DOI

http://dx.doi.org/10.1038/s41598-018-26933-0

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1104243699

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29855531


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