Role of cobalt cations in short range antiferromagnetic Co3O4 nanoparticles: a thermal treatment approach to affecting phonon and magnetic properties View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2018-12

AUTHORS

Swati R. Gawali, Ashish Chhaganlal Gandhi, Shrikrushna Shivaji Gaikwad, Jayashree Pant, Ting-Shan Chan, Chia-Liang Cheng, Yuan-Ron Ma, Sheng Yun Wu

ABSTRACT

We report the phonon and magnetic properties of various well-stabilized Co3O4 nanoparticles. The net valence in cobalt (II)/(III) cation can be obtained by subtracting the Co2+ ions in tetrahedral interstices and Co3+ ions in the octahedral interstices, respectively, which will possess spatial inhomogeneity of its magnetic moment via Co2+ in tetrahedra and Co3+ in octahedral configurations in the normal spinel structure. Furthermore, the distribution of Co2+/Co3+ governed by various external (magnetic field and temperature) and internal (particle size and slightly distorted CoO6 octahedra) sources, have led to phenomena such as a large redshift of phonon-phonon interaction and short-range magnetic correlation in the inverse spinel structure. The outcome of our study is important in terms of the future development of magnetic semiconductor spintronic devices of Co3O4. More... »

PAGES

249

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-017-18563-9

DOI

http://dx.doi.org/10.1038/s41598-017-18563-9

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1100203137

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29321560


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