Origin of methane-rich natural gas at the West Pacific convergent plate boundary View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2017-12

AUTHORS

Yuji Sano, Naoya Kinoshita, Takanori Kagoshima, Naoto Takahata, Susumu Sakata, Tomohiro Toki, Shinsuke Kawagucci, Amane Waseda, Tefang Lan, Hsinyi Wen, Ai-Ti Chen, Hsiaofen Lee, Tsanyao F. Yang, Guodong Zheng, Yama Tomonaga, Emilie Roulleau, Daniele L. Pinti

ABSTRACT

Methane emission from the geosphere is generally characterized by a radiocarbon-free signature and might preserve information on the deep carbon cycle on Earth. Here we report a clear relationship between the origin of methane-rich natural gases and the geodynamic setting of the West Pacific convergent plate boundary. Natural gases in the frontal arc basin (South Kanto gas fields, Northeast Japan) show a typical microbial signature with light carbon isotopes, high CH4/C2H6 and CH4/3He ratios. In the Akita-Niigata region - which corresponds to the slope stretching from the volcanic-arc to the back-arc -a thermogenic signature characterize the gases, with prevalence of heavy carbon isotopes, low CH4/C2H6 and CH4/3He ratios. Natural gases from mud volcanoes in South Taiwan at the collision zone show heavy carbon isotopes, middle CH4/C2H6 ratios and low CH4/3He ratios. On the other hand, those from the Tokara Islands situated on the volcanic front of Southwest Japan show the heaviest carbon isotopes, middle CH4/C2H6 ratios and the lowest CH4/3He ratios. The observed geochemical signatures of natural gases are clearly explained by a mixing of microbial, thermogenic and abiotic methane. An increasing contribution of abiotic methane towards more tectonically active regions of the plate boundary is suggested. More... »

PAGES

15646

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41598-017-15959-5

DOI

http://dx.doi.org/10.1038/s41598-017-15959-5

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1092622008

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/29142325


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