A quantum liquid of magnetic octupoles on the pyrochlore lattice View Full Text


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Article Info

DATE

2020-03-23

AUTHORS

Romain Sibille, Nicolas Gauthier, Elsa Lhotel, Victor Porée, Vladimir Pomjakushin, Russell A. Ewings, Toby G. Perring, Jacques Ollivier, Andrew Wildes, Clemens Ritter, Thomas C. Hansen, David A. Keen, Gøran J. Nilsen, Lukas Keller, Sylvain Petit, Tom Fennell

ABSTRACT

Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles1. Theories define such states using gauge fields and deconfined quasiparticle excitations that emerge from a local constraint governing the ground state of a frustrated magnet. For example, the ‘2-in–2-out’ ice rule for dipole moments on a tetrahedron can lead to a quantum spin ice2–4 in rare-earth pyrochlores. However, f-electron ions often carry multipole degrees of freedom of higher rank than dipoles, leading to intriguing behaviours and ‘hidden’ orders5,6. Here we show that the correlated ground state of a Ce3+-based pyrochlore, Ce2Sn2O7, is a quantum liquid of magnetic octupoles. Our neutron scattering results are consistent with a fluid-like state where degrees of freedom have a more complex magnetization density than that of magnetic dipoles. The nature and strength of the octupole–octupole couplings, together with the existence of a continuum of excitations attributed to spinons, provides further evidence for a quantum ice of octupoles governed by a ‘2-plus–2-minus’ rule7,8. Our work identifies Ce2Sn2O7 as a unique example of frustrated multipoles forming a ‘hidden’ topological order, thus generalizing observations on quantum spin liquids to multipolar phases that can support novel types of emergent fields and excitations. More... »

PAGES

546-552

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41567-020-0827-7

DOI

http://dx.doi.org/10.1038/s41567-020-0827-7

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1125824260

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/32802143


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78 scattering results
79 spin liquid
80 spinons
81 state
82 strength
83 such states
84 tetrahedra
85 theory
86 topological order
87 types
88 unique example
89 work
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