Two-dimensional spin liquid behaviour in the triangular-honeycomb antiferromagnet TbInO3 View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2019-03

AUTHORS

Lucy Clark, Gabriele Sala, Dalini D. Maharaj, Matthew B. Stone, Kevin S. Knight, Mark T. F. Telling, Xueyun Wang, Xianghan Xu, Jaewook Kim, Yanbin Li, Sang-Wook Cheong, Bruce D. Gaulin

ABSTRACT

Spin liquid ground states are predicted to arise within several distinct scenarios in condensed matter physics. The observation of these disordered magnetic states is particularly pervasive among a class of materials known as frustrated magnets, in which the competition between various magnetic exchange interactions prevents the system from adopting long-range magnetic order at low temperatures. Spin liquids continue to be of great interest due to their exotic nature and the possibility that they may support fractionalized excitations, such as Majorana fermions. Systems that allow for such phenomena are not only fascinating from a fundamental perspective but may also be practically significant in future technologies based on quantum computation. Here we show that the underlying antiferromagnetic sublattice in TbInO3 can undergo a crystal field-induced distortion of its buckled triangular arrangement to one based on a honeycomb. The absence of a conventional magnetic ordering transition at the lowest measurable temperatures indicates that another critical mechanism must govern in the ground-state selection of TbInO3. We suggest that anisotropic exchange interactions—mediated through strong spin–orbit coupling on the emergent honeycomb lattice of TbInO3—give rise to a highly frustrated spin liquid. Detailed neutron scattering, magnetic susceptibility and muon spin relaxation studies indicate the absence of long-range magnetic order in the quantum magnet TbInO3 down to 0.46 K— an observation consistent with quantum spin liquid behaviour. More... »

PAGES

262-268

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/s41567-018-0407-2

DOI

http://dx.doi.org/10.1038/s41567-018-0407-2

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111375502


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