Flexible layer-structured Bi2Te3 thermoelectric on a carbon nanotube scaffold View Full Text


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Article Info

DATE

2018-11-19

AUTHORS

Qun Jin, Song Jiang, Yang Zhao, Dong Wang, Jianhang Qiu, Dai-Ming Tang, Jun Tan, Dong-Ming Sun, Peng-Xiang Hou, Xing-Qiu Chen, Kaiping Tai, Ning Gao, Chang Liu, Hui-Ming Cheng, Xin Jiang

ABSTRACT

Inorganic chalcogenides are traditional high-performance thermoelectric materials. However, they suffer from intrinsic brittleness and it is very difficult to obtain materials with both high thermoelectric ability and good flexibility. Here, we report a flexible thermoelectric material comprising highly ordered Bi2Te3 nanocrystals anchored on a single-walled carbon nanotube (SWCNT) network, where a crystallographic relationship exists between the Bi2Te3 <[Formula: see text]> orientation and SWCNT bundle axis. This material has a power factor of ~1,600 μW m-1 K-2 at room temperature, decreasing to 1,100 μW m-1 K-2 at 473 K. With a low in-plane lattice thermal conductivity of 0.26 ± 0.03 W m-1 K-1, a maximum thermoelectric figure of merit (ZT) of 0.89 at room temperature is achieved, originating from a strong phonon scattering effect. The origin of the excellent flexibility and thermoelectric performance of the Bi2Te3-SWCNT material is attributed, by experimental and computational evidence, to its crystal orientation, interface and nanopore structure. Our results provide insight into the design and fabrication of high-performance flexible thermoelectric materials. More... »

PAGES

1-7

References to SciGraph publications

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  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1038/s41563-018-0217-z

    DOI

    http://dx.doi.org/10.1038/s41563-018-0217-z

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1109934342

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/30455446


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